Abstract-Optical Kerr nonlinearity and multi-photon absorption of DSTMS measured by Z-scan method

 

Jiang Li, Rakesh Rana, Liguo Zhu, Cangli Liu, Harald Schneider, Alexej Pashkin

 https://arxiv.org/abs/2102.03242

We investigate the optical Kerr nonlinearity and multi-photon absorption (MPA) properties of DSTMS excited by femtosecond pulses at a wavelengths of 1.43 {\mu}m, which is optimal for terahertz generation via difference frequency mixing. The MPA and the optical Kerr coefficients of DSTMS at 1.43 {\mu}m are strongly anisotropic indicating a dominating contribution from cascaded 2nd-order nonlinearity. These results suggest that the saturation of the THz generation efficiency is mainly related to the MPA process and to a spectral broadening caused by cascaded 2nd-order frequency mixing within DSTMS

Abstract-Non-plasmonic improvement in photoconductive THz emitters using nano- and micro-structured electrodes

 

Abhishek Singh, Malte Welsch, Stephan Winnerl, Manfred Helm, Harald Schneider, 

Simulation of electric field amplitude ((Ex2+Ey2+Ez2)1/2 in V/m) distribution on a slice passing through the center of the emitter in yz-plane in the photoconductor when 10 V bias is applied to the electrodes. Field lines are drawn to show the direction of the electric field. A white dashed line is drawn at a depth (∼ 1 µm) of penetration depth of 800 nm in GaAs.

https://www.osapublishing.org/oe/fulltext.cfm?uri=oe-28-24-35490&id=442489

We investigate here terahertz enhancement effects arising from micrometer and nanometer structured electrode features of photoconductive terahertz emitters. Nanostructured electrode based emitters utilizing the palsmonic effect are currently one of the hottest topics in the research field. We demonstrate here that even in the absence of any plasmonic resonance with the pump pulse, such structures can improve the antenna effect by enhancing the local d.c. electric field near the structure edges. Utilizing this effect in Hilbert-fractal and grating-like designs, enhancement of the THz field of up to a factor of ∼ 2 is observed. We conclude that the cause of this THz emission enhancement in our emitters is different from the earlier reported plasmonic-electrode effect in a similar grating-like structure. In our structure, the proximity of photoexcited carriers to the electrodes and local bias field enhancement close to the metallization cause the enhanced efficiency. Due to the nature of this effect, the THz emission efficiency is almost independent of the pump laser polarization. Compared to the plasmonic effect, these effects work under relaxed device fabrication and operating conditions.

Published by The Optical Society under the terms of the Creative Commons Attribution 4.0 License. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.

Abstract-Nonlinear Charge Transport in InGaAs Nanowires at Terahertz Frequencies

Rakesh Rana, Leila Balaghi, Ivan Fotev, Harald Schneider, Manfred Helm, Emmanouil Dimakis, Alexej Pashkin

https://arxiv.org/abs/2004.00484

We probe the electron transport properties in the shell of GaAs/In0.2Ga0.8As core/shell nanowires at high electric fields using optical pump / THz probe spectroscopy with broadband THz pulses and peak electric fields up to 0.6 MV/cm. The plasmon resonance of the photoexcited charge carriers exhibits a systematic redshift and a suppression of its spectral weight for THz driving fields exceeding 0.4 MV/cm. This behavior is attributed to the intervalley electron scattering resulting in the increase of the average electron effective mass and the corresponding decrease of the electron mobility by about 2 times at the highest fields. We demonstrate that the increase of the effective mass is non-uniform along the nanowires and takes place mainly in their middle part, leading to a spatially inhomogeneous carrier response. Our results quantify the nonlinear transport regime in GaAs-based nanowires and show their high potential for development of nano-devices operating at THz frequencies.

Abstract-Up to 70 THz bandwidth from an implanted Ge photoconductive antenna excited by a femtosecond Er:fibre laser

• Abhishek Singh, 
• Alexej Pashkin,  
• Stephan Winnerl, 
• Malte Welsch, 
• Cornelius Beckh, 
• Philipp Sulzer, 
• Alfred Leitenstorfer, 
• Manfred Helm,  
• Harald Schneider, 

Ultrabroadband THz emission from a Ge:Au antenna pumped at 1100 nm.

https://www.nature.com/articles/s41377-020-0265-4

Phase-stable electromagnetic pulses in the THz frequency range offer several unique capabilities in time-resolved spectroscopy. However, the diversity of their application is limited by the covered spectral bandwidth. In particular, the upper frequency limit of photoconductive emitters - the most widespread technique in THz spectroscopy – reaches only up to 7 THz in the regular transmission mode due to absorption by infrared-active optical phonons. Here, we present ultrabroadband (extending up to 70 THz) THz emission from an Au-implanted Ge emitter that is compatible with mode-locked fibre lasers operating at wavelengths of 1.1 and 1.55 μm with pulse repetition rates of 10 and 20 MHz, respectively. This result opens up the possibility for the development of compact THz photonic devices operating up to multi-THz frequencies that are compatible with Si CMOS technology.

Research team presents novel transmitter for terahertz waves

If a gallium-arsenide crystal is irradiated with short laser pulses, charge carriers are formed. These charges are accelerated by applying a voltage which enforces the generation of a terahertz wave. Credit: HZDR/Juniks

by Helmholtz Association of German Research Centres

https://phys.org/news/2020-03-team-transmitter-terahertz.html

Terahertz waves are becoming ever more important in science and technology. They enable us to unravel the properties of future materials, test the quality of automotive paint and screen envelopes. But generating these waves is still a challenge. A team at Helmholtz-Zentrum Dresden-Rossendorf (HZDR), TU Dresden and the University of Konstanz has now made significant progress. The researchers have developed a germanium component that generates short terahertz pulses with an advantageous property: the pulses have an extreme broadband spectrum and thus deliver many different terahertz frequencies at the same time. As it has been possible to manufacture the component employing methods already used in the semiconductor industry, the development promises a broad range of applications in research and technology, as the team reports in the journal Light: Science & Applications.

Just like light, terahertz waves are categorized as electromagnetic radiation. In the spectrum, they fall right between microwaves and infrared radiation. But while microwaves and infrared radiation have long since entered our everyday lives, terahertz waves are only just beginning to be used. The reason is that experts have only been able to construct reasonably acceptable sources for terahertz waves since the beginning of the 2000s. But these transmitters are still not perfect—they are relatively large and expensive, and the radiation they emit does not always have the desired properties.

One of the established generation methods is based on a gallium-arsenide crystal. If this semiconductor crystal is irradiated with short laser pulses, gallium arsenide charge carriers are formed. These charges are accelerated by applying voltage which enforces the generation of a terahertz wave—basically the same mechanism as in a VHF transmitter mast where moving charges produce radio waves.

However, this method has a number of drawbacks: "It can only be operated with relatively expensive special lasers," explains HZDR physicist Dr. Harald Schneider. "With standard lasers of the type we use for fiber-optic communications, it doesn't work." Another shortcoming is that gallium-arsenide crystals only deliver relatively narrowband terahertz pulses and thus a restricted frequency range—which significantly limits the application area.

Precious metal implants

That is why Schneider and his team are placing their bets on another material—the semiconductor germanium. "With germanium we can use less expensive lasers known as fiber lasers," says Schneider. "Besides, germanium crystals are very transparent and thus facilitate the emission of very broadband pulses." But, so far, they have had a problem: If you irradiate pure germanium with a short laser pulse, it takes several microseconds before the electrical charge in the semiconductor disappears. Only then can the crystal absorb the next laser pulse. Today's lasers, however, can fire off their pulses at intervals of a few dozen nanoseconds—a sequence of shots far too fast for germanium.

In order to overcome this difficulty, experts searched for a way of making the electrical charges in the germanium vanish more quickly. And they found the answer in a prominent precious metal—gold. "We used an ion accelerator to shoot gold atoms into a germanium crystal," explains Schneider's colleague, Dr. Abhishek Singh. "The gold penetrated the crystal to a depth of 100 nanometers." The scientists then heated the crystal for several hours at 900 degrees Celsius. The heat treatment ensured the gold atoms were evenly distributed in the germanium crystal.

Success kicked in when the team illuminated the peppered germanium with ultrashort laser pulses: instead of hanging around in the crystal for several microseconds, the electrical charge carriers disappeared again in under two nanoseconds—about thousand times faster than before. Figuratively speaking, the gold works like a trap, helping to catch and neutralize the charges. "Now the germanium crystal can be bombarded with laser pulses at a high repetition rate and still function," Singh is pleased to report.

Inexpensive manufacture possible

The new method facilitates terahertz pulses with an extremely broad bandwidth: instead of 7 terahertz using the established gallium-arsenide technique, it is now ten times greater—70 terahertz. "We get a broad, continuous, gapless spectrum in one fell swoop", Harald Schneider enthuses. "This means we have a really versatile source at hand that can be used for the most diverse applications." Another benefit is that, effectively, germanium components can be processed with the same technology that is used for microchips. "Unlike gallium arsenide, germanium is silicon compatible," Schneider notes. "And as the new components can be operated together with standard fiber-optic lasers, you could make the technology fairly compact and inexpensive."

This should turn gold-doped germanium into an interesting option not just for scientific applications, such as the detailed analysis of innovative two-dimensional materials such as graphene, but also for applications in medicine and environmental technology. One could imagine sensors, for instance, that trace certain gases in the atmosphere by means of their terahertz spectrum. Today's terahertz sources are still too expensive for the purpose. The new methods, developed in Dresden-Rossendorf, could help to make environmental sensors like this much cheaper in the future.

Abstract-Gapless broadband terahertz emission from a germanium photoconductive emitter

Abhishek Singh, Alexej Pashkin, Stephan Winnerl, Manfred Helm,  Harald Schneider

https://pubs.acs.org/doi/10.1021/acsphotonics.8b00460

Photoconductive terahertz (THz) emitters have been fulfilling many demands required for table-top THz time-domain spectroscopy up to 3-4 THz. In contrast to the widely used photoconductive materials such as GaAs and InGaAs, Ge is a non-polar semiconductor characterized by a gapless transmission in the THz region due to absence of one-phonon absorption. We present here the realization of a Ge-based photoconductive THz emitter with a smooth broadband spectrum extending up to 13 THz and compare its performance with a GaAs-based analogue. We show that the spectral bandwidth of the Ge emitter is limited mainly by the laser pulse width (65 fs) and, thus, can be potentially extended to even much higher THz frequencies.

Abstract-Terahertz dephasing of Landau level transitions in graphene

Harald Schneider, Jacob C. König-Otto,  Alexej Pashkin, Yongrui Wang, Alexey Belyanin, Manfred Helm,  Stephan Winnerl

http://ieeexplore.ieee.org/document/8066873/

Using degenerate four-wave mixing (DFWM), we have investigated the coherent polarization between the lowest Landau levels in graphene under resonant excitation with narrowband THz pulses. A pronounced DFWM signal is observed and its dependence on THz field strength and magnetic field detuning is explored and compared with theoretical expectations.

Abstract-Plasmonic efficiency enhancement at the anode of strip line photoconductive terahertz emitters

Abhishek Singh, Stephan Winnerl, Jacob C. König-Otto, Daniel R. Stephan, Manfred Helm, and Harald Schneider

https://www.blogger.com/blogger.g?blogID=124073320791841682#editor/target=post;postID=964173647966952561

We investigate strip line photoconductive terahertz (THz) emitters in a regime where both the direct emission of accelerated carriers in the semiconductor and the antenna-mediated emission from the strip line play a significant role. In particular, asymmetric strip line structures are studied. The widths of the two electrodes have been varied from 2 µm to 50 µm. The THz emission efficiency is observed to increase linearly with the width of the anode, which acts here as a plasmonic antenna giving rise to enhanced THz emission. In contrast, the cathode width does not play any significant role on THz emission efficiency.

© 2016 Optical Society of America

Full Article  |  PDF Article

Abstract-Gouy phase shift of a tightly focused, radially polarized beam

Korbinian J. Kaltnenecker, Jacob C. König-Otto, Martin Mittendorff, Stephan Winnerl, Harald Schneider, Manfred Helm, Hanspeter Helm, Markus Walther, and Bernd M. Fischer

https://www.osapublishing.org/optica/fulltext.cfm?uri=optica-3-1-35&id=335319

Radially polarized beams represent an important member of the family of vector beams, in particular due to the possibility of using them to create strong and tightly focused longitudinal fields, a fundamental property that has been exploited by applications ranging from microscopy to particle acceleration. Since the properties of such a focused beam are intimately related to the Gouy phase shift, proper knowledge of its behavior is crucial. Terahertz microscopic imaging is used to extract the Gouy phase shift of the transverse and longitudinal field components of a tightly focused, radially polarized beam. Since the applied terahertz time-domain approach is capable of mapping the amplitude and phase of an electromagnetic wave in space, we are able to directly trace the evolution of the geometric phase as the wave propagates through the focus. We observe a Gouy phase shift of 2𝜋 for the transverse and of 𝜋 for the longitudinal component. Our experimental procedure is universal and may be applied to determine the geometric phase of other vector beams, such as optical vortices, or even arbitrarily shaped and polarized propagating waves.

© 2016 Optical Society of America

Abstract-Plasmonic Superlensing in Doped GaAs

Markus Fehrenbacher , Stephan Winnerl , Harald Schneider , Jonathan Döring , Susanne C. Kehr ,Lukas M. Eng , Yongheng Huo , Oliver G. Schmidt ,Kan Yao , Yongmin Liu , and Manfred Helm

Nano Lett., Just Accepted Manuscript

DOI: 10.1021/nl503996q

Publication Date (Web): January 13, 2015

Copyright © 2015 American Chemical Society

http://pubs.acs.org/doi/abs/10.1021/nl503996q?journalCode=nalefd

We demonstrate a semiconductor based broadband near-field superlens in the mid-infrared regime. Here, the Drude response of a highly doped n-GaAs layer induces a resonant enhancement of evanescent waves accompanied by a significantly improved spatial resolution at radiation wavelengths around lambda=20um, adjustable by changing the doping concentration. In our experiments, gold stripes below the GaAs superlens are imaged with a lambda/6 sub-wavelength resolution by an apertureless near-field optical microscope utilizing infrared radiation from a free-electron laser. The resonant behavior of the observed superlensing effect is in excellent agreement with simulations based on the Drude-Lorentz model. Our results demonstrate a rather simple superlens implementation for infrared nanospectroscopy.