Showing posts with label Xi-Cheng Zhang. Show all posts
Showing posts with label Xi-Cheng Zhang. Show all posts

Wednesday, January 13, 2021

Abstract-Varying pre-plasma properties to boost terahertz wave generation in liquids

                                                        Communications Physics

Evgenia A. Ponomareva, Azat O. Ismagilov, Sergey E. Putilin, Anton N. Tsypkin, Sergei A. Kozlov,  Xi-Cheng Zhang,  

https://www.nature.com/articles/s42005-020-00511-1

Laser-driven nonlinear phenomena can both reveal the structural features of materials and become the basis for the development of various translated technologies, including highly intense terahertz sources. Here we realize a modified single-color double-pulse excitation scheme for enhancing the terahertz wave generation in flat liquid jets, and we show that the pre-ionization effect is crucial for finding the optimal input conditions. The experimental results, being supported by numerical simulations, reveal the preference for longer pre-pulses to induce the effective ionization process and shorter signals for the strong laser-plasma interaction. In addition to the identified features of the terahertz wave energy enhancement with respect to the duration change for both pulses and their ratio variation, we state the possibility of achieving the optical-to-THz conversion efficiency value up to 0.1% in the case of double-pulse excitation of an α-pinene jet.

Saturday, August 8, 2020

Abstract-Ultrafast hydrogen bond dynamics of liquid water revealed by terahertz-induced transient birefringence


Hang Zhao, Yong Tan, Liangliang Zhang, Rui Zhang, Mostafa Shalaby, Cunlin Zhang, Yuejin Zhao & Xi-Cheng Zhang
TKE measurement of liquid water.

https://www.nature.com/articles/s41377-020-00370-z

The fundamental properties of water molecules, such as their molecular polarizability, have not yet been clarified. The hydrogen bond network is generally considered to play an important role in the thermodynamic properties of water. The terahertz (THz) Kerr effect technique, as a novel tool, is expected to be useful in exploring the low-frequency molecular dynamics of liquid water. Here, we use an intense and ultrabroadband THz pulse (peak electric field strength of 14.9 MV/cm, centre frequency of 3.9 THz, and bandwidth of 1–10 THz) to resonantly excite intermolecular modes of liquid water. Bipolar THz field-induced transient birefringence signals are observed in a free-flowing water film. We propose a hydrogen bond harmonic oscillator model associated with the dielectric susceptibility and combine it with the Lorentz dynamic equation to investigate the intermolecular structure and dynamics of liquid water. We mainly decompose the bipolar signals into a positive signal caused by hydrogen bond stretching vibration and a negative signal caused by hydrogen bond bending vibration, indicating that the polarizability perturbation of water presents competing contributions under bending and stretching conditions. A Kerr coefficient equation related to the intermolecular modes of water is established. The ultrafast intermolecular hydrogen bond dynamics of water revealed by an ultrabroadband THz pump pulse can provide further insights into the transient structure of liquid water corresponding to the pertinent modes.

Sunday, June 14, 2020

Abstract-Ghost spintronic THz-emitter-array microscope


Si-Chao Chen, Zheng Feng, Jiang Li, Wei Tan, Liang-Hui Du, Jianwang Cai, Yuncan Ma, Kang He, Haifeng Ding, Zhao-Hui Zhai, Ze-Ren Li, Cheng-Wei Qiu, Xi-Cheng Zhang,  Li-Guo Zhu


https://www.nature.com/articles/s41377-020-0338-4

Terahertz (THz) waves show great potential in nondestructive testing, biodetection and cancer imaging. Despite recent progress in THz wave near-field probes/apertures enabling raster scanning of an object’s surface, an efficient, nonscanning, noninvasive, deep subdiffraction imaging technique remains challenging. Here, we demonstrate THz near-field microscopy using a reconfigurable spintronic THz emitter array (STEA) based on the computational ghost imaging principle. By illuminating an object with the reconfigurable STEA followed by computing the correlation, we can reconstruct an image of the object with deep subdiffraction resolution. By applying an external magnetic field, in-line polarization rotation of the THz wave is realized, making the fused image contrast polarization-free. Time-of-flight (TOF) measurements of coherent THz pulses further enable objects at different distances or depths to be resolved. The demonstrated ghost spintronic THz-emitter-array microscope (GHOSTEAM) is a radically novel imaging tool for THz near-field imaging, opening paradigm-shifting opportunities for nonintrusive label-free bioimaging in a broadband frequency range from 0.1 to 30 THz (namely, 3.3–1000 cm−1).

Saturday, May 2, 2020

Abstract-Preference of subpicosecond laser pulses for terahertz wave generation from liquids


Qi Jin,  Yiwen E,  Shenghan Gao,  Xi-Cheng Zhang,

https://www.spiedigitallibrary.org/journals/advanced-photonics/volume-2/issue-01/015001/Preference-of-subpicosecond-laser-pulses-for-terahertz-wave-generation-from/10.1117/1.AP.2.1.015001.full

Terahertz (THz) wave generation from laser-induced air plasma generally requires a short temporal laser pulse. In contrast, it was observed that THz radiation from ionized liquid water prefers a longer pulse, wherein the mechanism remains unclear. We attribute the preference for longer pulse duration to the process of ionization and plasma formation in water, which is supported by a numerical simulation result showing that the highest electron density is achieved with a subpicosecond pulse. The explanation is further verified by the coincidence of our experimental result and simulation when the thickness of the water is varied. Other liquids are also tested to assure the preference for such a pulse is not exclusive to water.

Wednesday, April 29, 2020

Making terahertz waves: Why liquids prefer long optical pulses


Original article published in Advanced Photonics. Credit: SPIE
https://phys.org/news/2020-04-terahertz-liquids-optical-pulses.html

Laser-induced ionization in matter—gas, cluster, liquid, and solid—occurs when a laser pulse with sufficient intensity is focused into a target material, creating electrons and ions through nonlinear processes of laser-matter interaction. Photoionization is an effective way to generate transient currents and electromagnetic radiation covering the spectrum from microwaves to X-rays.

In the terahertz (THz) , laser-induced air plasma has become one of the most popular THz sources in research labs. THZ generation from liquid water—long considered impossible—has been successfully demonstrated, with particular success from laser pulse repetitions targeting flowing liquid, so the chaos caused by the previous pulse does not influence the next.
Professor Xi-Cheng Zhang's group at University of Rochester's Institute of Optics conducts leading-edge research in THz wave generation from liquid water. They find that THz wave generation from ionized liquids involves photoionization processes that differ significantly from those of air or other gases. They discuss these differences in detail in a recent article published in Advanced Photonics.
Zhang's group observes that in gas, the shortest pulse always generates the strongest THz field, but in liquids, longer pulse duration offers stronger THz emission. By calculating the , they find that the longer pulse duration generates more electrons in liquid. According to their observations, this phenomenon is caused by the collision of electrons, which plays an important role in the ionization process. For gases, the lifetime of electrons is always longer than the pulse duration, so the collision effect is generally not considered.
The insight illuminates the influence of optical  duration on laser-induced ionization in THz wave generation and advances the development of  THz sources, rich in potential applications and opportunities.

Friday, July 12, 2019

Abstract-Strong Terahertz Radiation from a Liquid-Water Line


Liang-Liang Zhang, Wei-Min Wang, Tong Wu, Shi-Jia Feng, Kai Kang, Cun-Lin Zhang, Yan Zhang, Yu-Tong Li, Zheng-Ming Sheng, and Xi-Cheng Zhang
Figure
Terahertz radiation generation from liquid water has long been considered impossible due to strong absorption. A few very recent works reported terahertz generation from water, but the mechanism is not clear and the efficiency demands to be enhanced. We show experimentally that strong single-cycle terahertz radiation with field strength of 0.2MVcm1 is generated from a water line (or column) of approximately 200μm in diameter irradiated by a mJ femtosecond laser beam. This strength is 100-fold higher than that produced from air using single-color pumping. We attribute the mechanism to the laser-ponderomotive-force-induced current with the symmetry broken around the water-column interface. This mechanism can explain our following observations: the radiation can be generated only when the laser propagation axis deviates from the column center; the deviation determines its field strength and polarity; it is always p polarized no matter whether the laser is p or s polarized. This study provides a simple and efficient scheme of table-top terahertz sources based on liquid water.
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Sunday, June 23, 2019

Abstract-Spatial sampling of terahertz fields with sub-wavelength accuracy via probe-beam encoding


Jiapeng Zhao, Yiwen E, Kaia Williams, Xi-Cheng Zhang,  Robert W. Boyd, 

Fig. 1: Experimental Configuration
https://www.nature.com/articles/s41377-019-0166-6

Recently, computational sampling methods have been implemented to spatially characterize terahertz (THz) fields. Previous methods usually rely on either specialized THz devices such as THz spatial light modulators or complicated systems requiring assistance from photon-excited free carriers with high-speed synchronization among multiple optical beams. Here, by spatially encoding an 800-nm near-infrared (NIR) probe beam through the use of an optical SLM, we demonstrate a simple sampling approach that can probe THz fields with a single-pixel camera. This design does not require any dedicated THz devices, semiconductors or nanofilms to modulate THz fields. Using computational algorithms, we successfully measure 128 × 128 field distributions with a 62-μm transverse spatial resolution, which is 15 times smaller than the central wavelength of the THz signal (940 μm). Benefitting from the non-invasive nature of THz radiation and sub-wavelength resolution of our system, this simple approach can be used in applications such as biomedical sensing, inspection of flaws in industrial products, and so on.

Wednesday, May 29, 2019

Abstract-Flat liquid jet as a highly efficient source of terahertz radiation



Anton N. Tcypkin, Evgenia A. Ponomareva, Sergey E. Putilin, Semen V. Smirnov, Sviatoslav A. Shtumpf, Maksim V. Melnik, Yiwen E, Sergei A. Kozlov, and Xi-Cheng Zhang

Fig. 1 Experimental setup of terahertz generation in flat liquid jets. (a) Experimental layout for energy and spectral terahertz measurements (the inset shows an illustration of optical incident angle ϕ). Laser radiation is splat on pump and probe beams with beam-splitter (BS) with ratio of energy in the channels 1:49, for probe and pump, respectively. Parabolic mirror (PM1 with focal length equal 5 cm) focus the pump radiation on a liquid jet which leads to the generation of terahertz radiation asa result of filamentation inside ionizing liquid jet. The terahertz radiation is collected and collimated by TPX lens (TL) filtered by a teflon filter (F). For spectrum measurements we use conventional electro-optical system (EOS). Parabolic mirror (PM2 with focal length equal 12 cm) focus the terahertz radiation on the ZnTe crystal (EOC) with 1 mm thickness. (b) Photo of laser excitation of the liquid jet. Water moisture plum scatter the laser beam. Temporal terahertz signals (c) and spectrum (d) emitted from the jets of water and ethanol with a thickness of 150 μm at laser pulse duration of 400 fs and optical excitation energy of 600 μJ.

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-27-11-15485

Polar liquids are strong absorbers of electromagnetic waves in the terahertz range, therefore, historically such liquids have not been considered as good candidates for terahertz sources. However, flowing liquid medium has explicit advantages, such as a higher damage threshold compared to solid-state sources and more efficient ionization process compared to gases. Here we report systematic study of efficient generation of terahertz radiation in flat liquid jets under sub-picosecond single-color optical excitation. We demonstrate how medium parameters such as molecular density, ionization energy and linear absorption contribute to the terahertz emission from the flat liquid jets. Our simulation and experimental measurements reveal that the terahertz energy has quasi-quadratic dependence on the optical excitation pulse energy. Moreover, the optimal pump pulse duration, which depends on the thickness of the jet is theoretically predicted and experimentally confirmed. The obtained optical-to-terahertz energy conversion efficiency is more than 0.05%. It is comparable to the commonly used optical rectification in most of electro-optical crystals and two-color air filamentation. These results, significantly advancing prior research, can be successfully applied to create a new alternative source of terahertz radiation.
© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Sunday, April 14, 2019

Abstract-High Kerr nonlinearity of water in THz spectral range




Anton N. Tcypkin, Maksim V. Melnik, Maria O. Zhukova, Irina O. Vorontsova, Sergey E. Putilin, Sergei A. Kozlov, and Xi-Cheng Zhang

Fig. 1 (a) The experimental setup for measuring the nonlinear refractive index (n2) of a liquid jet in the THz spectral range. Two parabolic mirrors (PM1 and PM2) with a focal length of 12.5 mm form the caustics area where the water jet (jet) is scanned along the z axis. The synchronization is performed using the mechanical modulator (M) located between the lens and the Golay cell (GC). The aperture (A) is moved from open to closed position to change the geometry of Z-scan from open to closed aperture. Insert - Geometrical position of the jet moved along the z axis relative to the THz radiation. The temporal waveform (b) and its spectrum (c) of the THz pulse generated by the TERA-AX system.

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-27-8-10419

The values of the nonlinear refractive index coefficient for various materials in the terahertz frequency range exceed the ones in both visible and NIR ranges by several orders of magnitude. This allows to create nonlinear switches, modulators, systems requiring lower control energies in the terahertz frequency range. We report the direct measurement of the nonlinear refractive index coefficient of liquid water by using the Z-scan method with broadband pulsed THz beam. Our experimental result shows that nonlinear refractive index coefficient in water is positive and can be as large as 7×10−10 cm2/W in the THz frequency range, which exceeds the values for the visible and NIR ranges by 6 orders of magnitude. To estimate n2, we use the theoretical model that takes into account ionic vibrational contribution to the third-order susceptibility. We show that the origins of the nonlinearity observed are the anharmonicity of molecular vibrations.
© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Sunday, February 24, 2019

Abstract-Investigation of liquid lines as terahertz emitters under ultrashort optical excitation



Recently, there has been growing interest in terahertz (THz) wave generation from liquids under optical excitation. Here, we propose and demonstrate the use of liquid lines in place of liquid films as THz emitters to boost THz signals. The geometry of the emitter eliminates the total internal reflection at the flat liquid-air interface. In addition, we observe that the polarity of the liquid has a significant influence on the THz wave generation. Alpha-pinene, a nonpolar liquid, offers much stronger THz radiation than water does. Besides paving the way to develop intense liquid THz sources, our work indicates that THz waves could be a tool for the further study of laser-liquid interaction.

Sunday, January 27, 2019

Abstract-Spatial Sampling of Terahertz Fields with Sub-wavelength Accuracy via Probe Beam Encoding


Recently, computational sampling methods have been implemented to spatially characterize terahertz (THz) fields. Previous methods usually rely on either specialized THz devices such as THz spatial light modulators, or complicated systems requiring assistance from photon-excited free-carriers with high-speed synchronization among multiple optical beams. Here, by spatially encoding an 800 nm near-infrared (NIR) probe beam through the use of an optical SLM, we demonstrate a simple sampling approach that can probe THz fields with a single-pixel camera. This design does not require any dedicated THz devices, semiconductors or nanofilms to modulate THz fields. Through the use of computational algorithms, we successfully measure 128×128 field distributions with a 62 μm transverse spatial resolution, more than 15 times smaller than the central wavelength of the THz signal (940 μm). Benefitting from the non-invasive nature of THz radiation and sub-wavelength resolution of our system, this simple approach can be used in applications such as biomedical sensing, inspection of flaws. in industrial products, and so on.

Monday, December 31, 2018

Abstract-Terahertz wave emission from a liquid water film under the excitation of asymmetric optical fields

Publisher Logo


Qi Jin, Jianming Dai, Yiwen E, Xi-Cheng Zhang,

Schematic diagram of the experimental setup. A phase compensator (PC) is applied to control the relative phase between ω and 2ω pulses. DWP, dual-wavelength wave plate. PM, parabolic mirror with an effective focal length of 1-in

https://aip.scitation.org/doi/10.1063/1.5064644

Liquid water excited by intense two-color laser pulses radiates electromagnetic waves at terahertz frequencies. Compared with one-color excitation, two-orders of magnitude enhanced terahertz energy are observed by using asymmetric optical excitation with the same total excitation pulse energy and focusing geometry. Modulation of the terahertz field is achieved via the coherent control approach. We find that modulated and unmodulated terahertz energies have, respectively, quadratic and linear dependence on the laser pulse energy. This work, as part of terahertz aqueous photonics, paves an alternative way of studying laser-liquid interactions and developing intense terahertz sources.

Saturday, December 1, 2018

Terahertz Radiation in Liquids


                                       An experimental setup. CREDIT ITMO University
https://www.eurekalert.org/multimedia/pub/187251.php


A research team from ITMO University and the University of Rochester (the USA) conducted a study on the formation of terahertz radiation in liquids. Previously, the generation of such radiation in a liquid medium was considered impossible due to high absorption. However, in their new research, the scientists described this phenomenon's physical nature and demonstrated that liquid radiation sources can be equally effective to traditional ones. The results have been published in Applied Physics Letters.
Terahertz electromagnetic radiation can easily pass through most materials except metals and water. Today, it is widely used in security systems used to detect illicit drugs and weapons, as well as for biomedical research. Most modern research involving terahertz radiation focuses on finding new, more stable, powerful and efficient sources.
The most common sources of terahertz radiation are solid materials. In addition, there are sources based on femtosecond laser filamentation in air and gases. In this case, a powerful laser beam creates a plasma in the gas medium by ionizing it so that free electrons generate electromagnetic terahertz radiation. Although doing the same in a liquid medium was until now considered impossible due to high absorption, an international research team from ITMO University and the University of Rochester showed the opposite. Their new study revealed that liquid, in fact, has a number of advantages over other sources such as gases.
"Until our colleague, Prof. Xi-Cheng Zhang, had been able to detect terahertz radiation in a liquid, it was believed to be impossible. But we demonstrated that, in terms of efficiency, liquid sources can approach solid-state sources, which are now considered to be the standard. Moreover, liquids are much easier to obtain than crystals. They can also withstand high pumping energy, which makes it possible to obtain a better output," explains Anton Tsypkin, Head of the Laboratory of Femtosecond Optics and Femtotechnology at ITMO University.
Usually, radiation is generated due to the release of free excited electrons during filamentation. The more electrons can be excited or ionized, the stronger the output terahertz radiation will be. The number of excited electrons of one molecule depends on the energy spent on the excitation or "pumping" of the medium. The difference between the required "pumping" energies in gas and liquid is small. At the same time, the density of molecules in a liquid is much higher than in a gas, so that a comparable pump energy makes it possible to excite more electrons and make the radiation stronger.
Scientists investigated the direction of terahertz radiation in the liquid. Experiments were conducted in parallel at two universities so as to eliminate errors. Then, the scientists verified the independently obtained results and worked together on a theoretical model to explain them. As a result, they managed to draw up and physically substantiate the radiation patterns of terahertz radiation in a liquid and its dependence on the angle at which the liquid collides with the pump radiation. According to the researchers, these results will be used in future work.
"A significant drawback of fluid is its large absorption. We plan to solve this problem by optimizing the type of fluid, the shape of the jet, the pump power and a number of other parameters. We want to experimentally find the optimal parameters for the radiation generation in different liquids, as well as to develop a theoretical model based on this data. It can be used to create a prototype device that will allow us to produce different types of terahertz radiation from liquids," says Xi-Cheng Zhang, co-director of the International Institute "Photonics and Optical Informatics" at ITMO University, and a researcher at the University of Rochester.
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Reference:
"Terahertz wave generation from liquid water films via laser-induced breakdown" 
Yiwen E, Qi Jin, Anton Tcypkin, and X.-C. Zhang. 
Appl. Phys. Lett. Nov. 1, 2018
Disclaimer: AAAS and EurekAlert! are not responsi

Wednesday, August 1, 2018

Abstract-Wireless Data Transmission Method Using Pulsed THz Sliced Spectral Supercontinuum



Yaroslav V. Grachev,  Xinrui Liu, Sergey E. Putilin,  Anton N. Tsypkin,   Victor G. Bespalov,  Sergei A. Kozlov, Xi-Cheng Zhang

https://ieeexplore.ieee.org/document/8119558/

A method of ultrafast wireless information transmission using spectrum-sliced supercontinuum (SC) along the THz frequency range is presented in this letter. The THz spectrum-sliced SC was formed by femtosecond optical pulses doubled in a Michelson interferometer before being input onto a MgO:LiNbO3-THz generator. Two THz pulses generated by femtosecond pulses within a MgO:LiNbO3-crystal provided the spectrum-sliced SC in the spectral domain, which was recorded by an electro-optical detection system. The transmission rate in this method is determined by the bandwidth of the THz spectrum, the number of spectral lines in the SC, and the pulse repetition rate. We have demonstrated an SC containing 31 spectral lines with 23-GHz spacing within the range from 0.04 to 0.75 THz. The signal with encoded information was successfully transmitted over 2.4 m in free-space.

Wednesday, December 20, 2017

Abstract-Wireless data transmission method using pulsed THz sliced spectral supercontinuum



 Yaroslav V. Grachev,  Xinrui Liu, Sergey E. Putilin, Anton N. Tsypkin,   Victor G. Bespalov,  Sergei A. Kozlov,   Xi-Cheng Zhang


A method of ultrafast wireless information transmission using spectrum-sliced supercontinuum (SC) along the THz frequency range is presented in this manuscript. The THz spectrum-sliced SC was formed by femtosecond optical pulses doubled in a Michelson interferometer before being input onto a MgO:LiNbO3 THz generator. Two THz pulses generated by femtosecond pulses within a MgO:LiNbO3 crystal provided the spectrum-sliced SC in the spectral domain, which was recorded by an electro-optical detection system. The transmission rate in this method is determined by the bandwidth of the THz spectrum, the number of spectral lines in the SC, and the pulse repetition rate. We have demonstrated a SC containing 31 spectral lines with 23 GHz spacing within the range from 0.04 to 0.75 THz. The signal with encoded information was successfully transmitted over 2.4 meters in free-space.

Saturday, September 30, 2017

Generating terahertz radiation from water makes ‘the impossible, possible’



Researchers use lasers to generate terahertz pulses via interaction with a target. In this case, the target was an extremely thin water film—approximately 200 microns or about the thickness of two pieces of paper—created using water suspended between two aluminum wires. (University of Rochester photo / Kaia Williams)

http://www.rochester.edu/newscenter/generating-terahertz-radiation-from-water-makes-the-impossible-possible-271292/

Xi-Cheng Zhang has worked for nearly a decade to solve a scientific puzzle that many in the research community believed to be impossible: producing terahertz waves—a form of electromagnetic radiation in the far infrared frequency range—from liquid water.
Now, as reported in a paper published in Applied Physics Letters, researchers at the University of Rochester have “made the impossible, possible,” says Zhang, the M. Parker Givens Professor of Optics. “Figuring out how to generate terahertz waves from liquid water is a fundamental breakthrough because water is such an important element in the human body and on Earth.”
Terahertz waves have attracted increased attention recently because of their ability to nondestructively pass through solid objects, including those made of cloth, paper, wood, plastic, and ceramics, and produce images of the interiors of the objects. Additionally, the energy of a terahertz photon is weaker than an x-ray photon. Unlike x-rays, terahertz waves are non-ionizing—they do not have enough energy to remove an electron from an atom—so they do not have the same harmful effects on human tissue and DNA.
Because of these abilities, terahertz waves have unique applications in imaging and spectroscopy—everything from discovering bombs in suspicious packages, to identifying murals hidden beneath coats of paint, to detecting tooth decay.
“Terahertz waves have a capacity to see through clothing, which is why you have these sub-terahertz body scanners at airports,” Zhang says. “These waves can help to identify if an object is explosive, chemical, or biological, even if they can’t tell exactly what the object is.”
Zhang’s research group uses lasers to generate terahertz pulses via interaction with a target. In this case, the target is an extremely thin film of water—approximately 200 microns or about the thickness of two pieces of paper—created using water suspended by surface tension between two aluminum wires. Researchers focus a laser into the water film, which acts as an emitter for the terahertz radiation output.
scientific diagram showing a pump beam going through a water film
The experimental set-up used to generate terahertz waves from liquid water. Researchers focus the optical pump beam into the water film and use a series of filters and off-axis parabolic mirrors (OAPMs) to detect the terahertz signal and block any other light waves simultaneously generated from the water film.
Previous researchers have generated terahertz waves from targets of solid crystals, metals, air plasma, and water vapor, but, until now, liquid water has proved elusive.
“Water was considered the enemy of terahertz waves because of water’s strong absorption,” Zhang says. “We always tried to avoid water, but it is a surprisingly efficient terahertz source.”
In fact, when researchers measured the terahertz waves generated by the water, they found they were 1.8 times stronger than the terahertz waves generated from air plasma under comparable experimental conditions.
Because water is such a strong absorber, however, many people in the research community believed it would be impossible to use water as a target. Zhang himself has spent years attempting a solution, and he found a likewise stalwart in Qi Jin, now a PhD candidate in optics at Rochester, and the lead author on the paper.
“Almost everybody thought we wouldn’t be able to get a signal from water,” Jin says. “At first, I didn’t believe it either.”
One of the challenges was creating a film of water thin enough that the terahertz photons generated by the laser beam would not be absorbed, but thick enough to withstand the laser’s energy.
Along with Yiwen E, a postdoctoral associate in Zhang’s research group, Jin spent months optimizing the thickness of the water film and the incident angle, intensity, and pulse duration of the laser beam.
“We increased the thickness of the water a little bit, and gradually increased the laser, and just kept trying until we could make it work,” Jin says.  “Water is one of the richest resources on Earth, so it was really important for us to be able to generate these waves from water. There were many times I wanted to give up on this, but people in the lab kept encouraging me.”
Zhang agrees: “I always tell my students and researchers here: if you try something, you might not get the result you wanted. But if you never try it, you definitely won’t get it.”
The research was sponsored by grants from the Army Research Office.