Showing posts with label Costas M. Soukoulis. Show all posts
Showing posts with label Costas M. Soukoulis. Show all posts

Wednesday, March 13, 2019

Abstract-Nonlinearity in the Dark: Broadband Terahertz Generation with Extremely High Efficiency



Ming Fang, Nian-Hai Shen, Wei E. I. Sha, Zhixiang Huang, Thomas Koschny, and Costas M. Soukoulis

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https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.122.027401

Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order nonlinear applications encounter fundamental trade-offs in the necessary symmetry breaking and local-field enhancement due to radiation damping that is inherent to the operating resonant mode and cannot be controlled separately. Here we present a novel concept that eliminates this restriction obstructing the improvement of terahertz generation efficiency in nonlinear metasurfaces based on metallic nanoresonators. This is achieved by combining a resonant dark-state metasurface, which locally drives nonlinear nanoresonators in the near field, with a specific spatial symmetry that enables destructive interference of the radiating linear moments of the nanoresonators, and perfect absorption via simultaneous electric and magnetic critical coupling of the pump radiation to the dark mode. Our proposal allows eliminating linear radiation damping, while maintaining constructive interference and effective radiation of the nonlinear components. We numerically demonstrate a giant second-order nonlinear susceptibility ∼10−11  m/V, a one order improvement compared with the previously reported split-ring-resonator metasurface, and correspondingly, a 2 orders of magnitude enhanced terahertz energy extraction should be expected with our configuration under the same conditions. Our study offers a paradigm of high efficiency tunable nonlinear metadevices and paves the way to revolutionary terahertz technologies and optoelectronic nanocircuitry.
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Saturday, June 2, 2018

Abstract-Investigation of broadband terahertz generation from metasurface




https://www.osapublishing.org/oe/fulltext.cfm?uri=oe-26-11-14241

The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single layer nanoscale split-ring resonator array. The terahertz generation due to optical rectification by the second-order nonlinearity of the split-ring resonator is investigated by a time-domain implementation of the hydrodynamic model for electron dynamics in metal. The results show that the nonlinear metasurface enables us to generate broadband terahertz radiation and free from quasi-phase-matching conditions. The proposed scheme provides a new concept of broadband THz source and designing nonlinear plasmonic metamaterials.
© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Sunday, June 11, 2017

Abstract-Photo-imprinted controllable Fano resonance in the terahertz regime


Giorgos Georgiou, Nian-Hai Shen, Jaime Gómez-Rivas, Thomas Koschny, and Costas M. Soukoulis

http://cdn-pubs.acs.org/doi/abs/10.1021/acsphotonics.7b00372

The emergence of metamaterials, including the recently proposed metasurfaces, provides unprecedented opportunities in the manipulation as well as the generation of terahertz (THz) waves. Various actively controllable THz devices such as optical switches and phase modulators have been achieved by incorporating external-stimuli-responsive media (typically semiconductors) in the configurations. Compared to pre-designed metallic-resonator-based metamaterials, photo-imprinted photonic structures offer us an all-optical route toward reconfigurable functionalities with superior flexibility. Here, we propose to photo-imprint some specific patterns on a thin film of semiconductor to excite Fano-like resonances, which result from the coupling between dark and bright elements. Experimental measurements, performed with THz time-domain spectroscopy, demonstrate counterintuitive tunable deep features in extinction spectra positioned around the expected resonance frequency. Our simulations are in excellent agreement with the experiments, by resembling realistic conditions of low contrast photo-imprinted patterns generated with a spatial light modulator and a finite detection time window. This work takes the first step toward realizing switchable Fano resonances via an all-optical approach, and therefore paves the way to more versatile manipulations of THz waves.

Thursday, August 11, 2016

Iowa State Physicists Win W.M. Keck Foundation Grant To Develop Terahertz Nanoscope

http://www.publicnow.com/view/7C85525E85A1BFCC59F34B952BF85C496329DB61

AMES, Iowa - Researchers from Iowa State University's department ofphysics and astronomy are working to build a powerful instrument capable of exploring and tuning materials in ways that could help solve the world's energy, information processing and data storage needs.
The researchers call their proposed instrument an extreme quantum terahertz nanoscope. Its primary function will be to discover materials and material functions at unprecedented scales of space, time and energy, enabling studies at scales that are ultrafast, ultrasmall and at very low frequency. The instrument will also allow researchers to control the materials they study.
'We want to develop a microscope that doesn't exist yet,' said Jigang Wang, the project leader, an Iowa State associate professor of physics and astronomy and an associate of the U.S. Department of Energy's Ames Laboratory. 'We're trying to see new things by looking across these three dimensions simultaneously. We want to understand how the electrons move and communicate in order to produce fascinating properties of materials.
'All of this will create a new paradigm to understand materials, control their properties and have far-reaching consequences to promote science and future technology.'
The W.M. Keck Foundation of Los Angeles - one of the country's largest philanthropic organizations - recently awarded a three-year, $1.3 million grant to support construction, commissioning and initial use of the nanoscope. The project will be known as the W.M. Keck Initiative in Ultrafast Quantum Microscopy of Emergent Orders.
Iowa State is also supporting the project with funds from the Office of the Vice President for Research, the College of Liberal Arts and Sciences and the department of physics and astronomy. And the Ames Laboratory is supporting the project with specialized laboratory space in the laboratory's new Sensitive Instrument Facility.
The grant was made through the Iowa State University Foundation, a private, nonprofit corporation dedicated to securing and managing gifts and grants that benefit Iowa State.
A diverse team and extreme scales
Wang said the quantum nanoscope project was made possible by the expertise, technical resources and close collaboration of Iowa State and Ames Laboratory scientists. The project team includes:
  • Wang who has expertise in ultra-fast optics and terahertz spectroscopy of complex materials.
  • Zhe Fei, an Iowa State assistant professor of physics and astronomy and an Ames Laboratory associate, who has expertise in scanning near-field optical microscopy.
  • Paul C. Canfield, an Iowa State Distinguished Professor of physics and astronomy and an Ames Laboratory senior physicist, who has expertise in new materials design and discovery.
  • Costas Soukoulis, an Iowa State Distinguished Professor of physics and astronomy and an Ames Laboratory senior physicist, and Thomas Koschny, an Ames Laboratory associate scientist, who have expertise in plasmonics, the study of light waves and metal surfaces, and metamaterials, materials with properties not found in nature.
Wang said the researchers will work together to develop a nanoscope that collects data at three extreme scales: billionths of a meter in space (nanometers), quadrillionths of a second in time (femtoseconds) and thousandths of electron volts in energy (milli-electron volts or terahertz).
He said each of those three dimensions - space, time and energy - is like the side of a triangle.
'On each side of that triangle humanity has achieved tremendous progress and understanding,' he said. 'But what about the region on the inside of the triangle, this inaccessible region that combines the best of all three fields? For many outstanding scientific and technological problems, our answers are largely limited by our inability to see inside this region. Through this award from the Keck Foundation, this instrument we're building will break down the barriers and allow us to see what's there.'
When the instrument's superconducting magnet, scanning near field microscopy probes, ultrafast lasers and other components are assembled, Wang said the nanoscope will be commissioned by studying graphene, a thin layer of carbon atoms packed in a honeycomb. The instrument's initial experiments will study a high-temperature, iron-based superconductor, a material that can conduct electricity with no resistance and support exotic magnetic properties when cooling in a fashion different from conventional metals.
The researchers will also experiment with using the nanoscope to manipulate electrons so they can tune materials with minimal heating of the samples. Study goals include discovering new states of matter and establishing the shortest times and smallest lengths for these states to switch.
The researchers wrote that they expect the nanoscope and its measurements to 'reveal the secrets of emergent-order phenomena and manipulate them at will, a monumental challenge in this age of novel materials.'
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Based in Los Angeles, the W. M. Keck Foundation was established in 1954 by the late W. M. Keck, founder of the Superior Oil Company. The Foundation's grant making is focused primarily on pioneering efforts in the areas of medical, science and engineering research. The Foundation also maintains an undergraduate education program that promotes distinctive learning and research experiences for students in the sciences and in the liberal arts, and a Southern California Grant Program that provides support for the Los Angeles community, with a special emphasis on children and youth from low-income families, special needs populations and safety-net services. For more information, please visitwww.wmkeck.org.

Saturday, July 16, 2016

Abstract-Electrically Tunable Goos–Hänchen Effect with Graphene in the Terahertz Regime



  1. Yuancheng Fan1,*, 
  2. Nian-Hai Shen2, 
  3. Fuli Zhang1, 
  4. Zeyong Wei3, 
  5. Hongqiang Li3,
  6. Qian Zhao4, 
  7. Quanhong Fu1, 
  8. Peng Zhang2,
  9. Thomas Koschny2 and
  10. Costas M. Soukoulis2,5
Version of Record online: 14 JUL 2016
DOI: 10.1002/adom.201600303

Goos–Hänchen (G–H) effect is of great interest in the manipulation of optical beams. However, it is still fairly challenging to attain efficient controls of the G–H shift for diverse applications. Here, a mechanism to realize tunable G–H shift in the terahertz regime with electrically controllable graphene is proposed. Taking monolayer graphene covered epsilon-near-zero metamaterial as a planar model system, it is found that the G–H shifts for the orthogonal s-polarized and p-polarized terahertz beams at oblique incidence are positive and negative, respectively. The G–H shift can be modified substantially by electrically controlling the Fermi energy of the monolayer graphene. Reversely, the Fermi energy dependent G–H effect can also be used as a strategy for measuring the doping level of graphene. In addition, the G–H shifts of the system are of strong frequency-dependence at oblique angles of incidence, therefore the proposed graphene hybrid system can potentially be used for the generation of terahertz “rainbow,” a flat analog of the dispersive prism in optics. The proposed scheme of hybrid system involving graphene for dynamic control of G–H shift will have potential applications in the manipulation of terahertz waves.

Wednesday, April 8, 2015

Abstract-Tunable terahertz frequency comb generation using time-dependent graphene sheets


Vincent Ginis, Philippe Tassin, Thomas Koschny, and Costas M. Soukoulis
Phys. Rev. B 91, 161403(R) – Published 8 April 2015

We investigate the interaction between electromagnetic pulses and two-dimensional current sheets whose conductivity is controlled as a function of time by the generation of photocarriers, and we discuss its applicability to tunable frequency comb generation. To this aim, we develop an analytical model that permits the calculation of the scattered waves off a thin sheet with time-dependent, dispersive sheet conductivity. We evaluate the transmitted spectrum as a function of the dispersive behavior and the modulation frequency of the number of photocarriers. We conclude that such active materials, e.g., time-dependent graphene sheets, open up the possibility to manipulate the frequency of incident pulses and, hence, could lead to highly tunable, miniaturized frequency comb generation.


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    Friday, February 27, 2015

    Metamaterials Shine Bright as New Terahertz Source

    Discovery demonstrates how metamaterials may be used in non-invasive material imaging and sensing, and terahertz information technologies.

    Click to enlarge photo. Enlarge Photo
    Image courtesy of Ames Laboratory
    A metamaterial that consists of a two-dimensional array of U-shaped gold structures (square background in the picture) efficiently emits terahertz frequency electromagnetic waves (red axis) when illuminated by a wavelength tunable near-infrared pump laser (blue axis).


    The Science

    Metamaterials allow design and use of light-matter interactions at a fundamental level. An efficient terahertz emission from two-dimensional arrays of gold split-ring resonator metamaterials was discovered as a result of excitation by a near-infrared pulsed laser.

    The Impact

    Terahertz waves are used in non-invasive imaging and sensing technology, in addition to information, communication, processing, and data storage technologies. Despite their widely recognized importance, however, there are few terahertz sources presently available due to the limitations of natural materials. This discovery opens new ways to use metamaterials for these important applications.

    Summary

    Broadband terahertz sources offer exciting possibilities to study fundamental physics principles, to develop non-invasive material imaging and sensing, and make possible terahertz information, communication, processing, and storage. The terahertz spectral range sits between infrared and typical radar frequencies, and the challenges of efficiently generating and detecting terahertz radiation has limited its use. To solve these challenges consider metamaterials; materials that allow control of the properties of light-matter interactions at the fundamental level. The building blocks of metamaterials, known as split-ring resonators, can be designed to exhibit strong electric and magnetic response to electromagnetic fields over a wide frequency range, from terahertz to infrared. Scientists at Ames Laboratory, Iowa State University, and Karlsruhe Institute of Technology in Germany have discovered that when a two-dimensional array of nanometer-sized gold metamaterial resonators is illuminated by a tunable near-infrared femtosecond laser, with wavelengths matching the magnetic resonance of the metamaterial, a strong broadband of terahertz electromagnetic waves is emitted. The efficiency of this conversion to terahertz waves was significantly better than conventional materials that are presently used for these applications. Detailed analysis of the directionality and polarization of the emitted radiation reveals the fundamental nature of this efficient wavelength conversion. Further, these new metamaterials could allow integration of terahertz optoelectronics with high-speed telecommunications.

    Contact

    Costas M. Soukoulis 
    Ames Laboratory
    soukoulis@ameslab.gov

    Funding

    DOE Office of Science, Basic Energy Sciences (experiments). Theory research was supported by the US Office of Naval Research and the National Science Foundation. The Karlsruhe team had support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation), the State of Baden-Wurttemberg, and the Karlsruhe Institute of Technology (KIT) through the DFG-Center for Functional Nanostructures (CFN).

    Publications

    L. Luo, I. Chatzakis, J. Wang, F.B. P. Niesler, M. Wegener, T. Koschny, C.M. Soukoulis, "Broadband terahertz generation from metamaterials," Nature Communications 5, 3055, 2014. [DOI: 10.1038/ncomms4055]

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    Program: BES, MSE
    Performer/Facility: University, DOE Laboratory

    Tuesday, September 30, 2014

    Abstract-Comparison of gold- and graphene-based resonant nanostructures for terahertz metamaterials and an ultrathin graphene-based modulator


    Nian-Hai Shen, Philippe Tassin, Thomas Koschny, and Costas M. Soukoulis

    https://journals.aps.org/prb/abstract/10.1103/PhysRevB.90.115437


    Graphene exhibits unique material properties, and in electromagnetic wave technology it raises the prospect of devices miniaturized down to the atomic length scale. Here we study split-ring resonator metamaterials made from graphene and we compare them to gold-based metamaterials. We find that graphene's huge reactive response derived from its large kinetic inductance allows for deeply subwavelength resonances, although its resonance strength is reduced due to higher dissipative loss damping and smaller dipole coupling. Nevertheless, tightly stacked graphene rings may provide for negative permeability and the electric dipole resonance of graphene meta-atoms turns out to be surprisingly strong. Based on these findings, we present a terahertz modulator based on a metamaterial with a multilayer stack of alternating patterned graphene sheets separated by dielectric spacers. Neighboring graphene flakes are biased against each other, resulting in modulation depths of over 75% at a transmission level of around 90%.
    DOI: http://dx.doi.org/10.1103/PhysRevB.90.115437
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    ©2014 American Physical Society

    Friday, January 17, 2014

    Highly efficient broadband terahertz radiation from metamaterials


    A THz spectrometer driven by femtosecond laser pulses was used to demonstrate THz emission from a split-ring resonator metamaterial of single nanometer thickness
     http://phys.org/news/2014-01-highly-efficient-broadband-terahertz-metamaterials.html#jCp
    by Breehan Gerleman Lucchesi

    (Phys.org) —Scientists at the U.S. Department of Energy's Ames Laboratory have demonstrated broadband terahertz (THz) wave generation using metamaterials. The discovery may help develop noninvasive imaging and sensing, and make possible THz-speed information communication, processing and storage. The results appeared in the Jan. 8 issue of Nature Communications.

    Terahertz electromagnetic waves occupy a middle ground between electronics waves, like microwave and radio waves, and photonics waves, such as infrared and UV waves. Potentially, THz waves may accelerate telecom technologies and break new ground in understanding the fundamental properties of photonics. Challenges related to efficiently generating and detecting THz waves has primarily limited their use.
    Traditional methods seek to either compress oscillating waves from the electronic range or stretch waves from the optical range. But when compressing waves, the THz frequency becomes too high to be generated and detected by conventional electronic devices. So, this approach normally requires either a large-scale electron accelerator facility or highly electrically-biased photoconductive antennas that produce only a narrow range of waves.
    To stretch optical waves, most techniques include mixing two laser frequencies inside an inorganic or organic crystal. However, the natural properties of these crystals result in low efficiency.
    So, to address these challenges, the Ames Laboratory team looked outside natural materials for a possible solution. They used man-made materials called metamaterials, which exhibit optical and magnetic properties not found in nature.
    Costas Soukoulis, an Ames Laboratory physicist and expert in designing metamaterials, along with collaborators at Karlsruhe Institute of Technology in Germany, created a metamaterial made up of a special type of meta-atom called split-ring resonators. Split-ring resonators, because of their u-shaped design, display a strong magnetic response to any desired frequency waves in the THz to infrared spectrum.


    A team led by Ames Laboratory physicists demonstrated broadband, gapless terahertz emission (red line) from split-ring resonator metamaterials (background) in the telecomm wavelength. The THz emission spectra exhibit significant enhancement at magnetic-dipole resonance of the metamaterials emitter (shown in inset image). This approach has potential to generate gapless spectrum covering the entire THz band, which is key to developing practical THz technologies and to exploring fundamental understanding of optics.

    Ames Laboratory physicist Jigang Wang, who specializes in ultra-fast laser spectroscopy, designed the femto-second laser experiment to demonstrate THz emission from the metamaterial of a single nanometer thickness.
    "The combination of ultra-short laser pulses with the unique and unusual properties of the metamaterial generates efficient and broadband THz waves from emitters of significantly reduced thickness," says Wang, who is also an associate professor of Physics and Astronomy at Iowa State University.
    The team demonstrated their technique using the wavelength used by telecommunications (1.5 microns), but Wang says that the THz generation can be tailored simply by tuning the size of the meta-atoms in the metamaterial.
    "In principle, we can expand this technique to cover the entire THz range," said Soukoulis, who is also a Distinguished Professor of physics and astronomy at Iowa State University.
    What's more, the team's metamaterial THz emitter measured only 40 nanometers and performed as well as traditional emitters that are thousands of times thicker.
    "Our approach provides a potential solution to bridge the 'THz technology gap' by solving the four key challenges in the THz emitter technology: efficiency; broadband spectrum; compact size; and tunability," said Wang.
    Soukoulis, Wang, Liang Luo and Thomas Koschny's work at Ames Laboratory was supported by the U.S. Department of Energy's Office of Science. Wang's work is partially supported by Ames Laboratory's Laboratory Directed Research and Development (LDRD) funding.
    DOE's Office of Science is the single largest supporter of basic research in the physical sciences in the United States, and is working to address some of the most pressing challenges of our time. For more information, please visit the Office of Science website at science.energy.gov/.
    Ames Laboratory is a U.S. Department of Energy Office of Science national laboratory operated by Iowa State University. Ames Laboratory creates innovative materials, technologies and energy solutions. We use our expertise, unique capabilities and interdisciplinary collaborations to solve global problems.

    More information: "Broadband terahertz generation from metamaterials." Liang Luo, Ioannis Chatzakis, Jigang Wang, Fabian B. P. Niesler, Martin Wegener, Thomas Koschny, Costas M. Soukoulis. Nature Communications 5, Article number: 3055 DOI: 10.1038/ncomms4055. Received 05 August 2013 Accepted 03 December 2013 Published 08 January 2014


    Wednesday, January 8, 2014

    Abstract-Broadband terahertz generation from metamaterials


    http://www.nature.com/ncomms/2014/140108/ncomms4055/full/ncomms4055.html

    The terahertz spectral regime, ranging from about 0.1–15 THz, is one of the least explored yet most technologically transformative spectral regions. One current challenge is to develop efficient and compact terahertz emitters/detectors with a broadband and gapless spectrum that can be tailored for various pump photon energies. Here we demonstrate efficient single-cycle broadband THz generation, ranging from about 0.1–4 THz, from a thin layer of split-ring resonators with few tens of nanometers thickness by pumping at the telecommunications wavelength of 1.5 μm (200 THz). The terahertz emission arises from exciting the magnetic-dipole resonance of the split-ring resonators and quickly decreases under off-resonance pumping. This, together with pump polarization dependence and power scaling of the terahertz emission, identifies the role of optically induced nonlinear currents in split-ring resonators. We also reveal a giant sheet nonlinear susceptibility ~10−16 m2 V−1 that far exceeds thin films and bulk non-centrosymmetric materials.