Lipeng Zhu, Zehan Yao, Yuanyuan Huang, Chuan He, Baogang Quan, Junjie Li, Changzhi Gu, Xinlong Xu, and Zhaoyu Ren
https://journals.aps.org/prapplied/abstract/10.1103/PhysRevApplied.12.044063
Circular photon drag effect (CPDE) is important for helicity-dependent optoelectronic emitters and detectors yet is less studied in graphene due to the relatively weak light-matter interaction and is submerged by other nonlinear optical effects. We give experimental evidence of CPDE in vertically grown graphene (VGG) by terahertz (THz) emission spectroscopy. The emitted THz polarization states can be tuned to linear, left-handed, and right-handed elliptical polarizations by changing the helicity of the pump laser. Polarity reversal of the THz time-domain signal occurs with the opposite helicity of pump laser excitation due to the CPDE. Theory analysis suggests that both the linear photon drag effect and CPDE-induced transient photocurrents contribute to the THz emission from which the contribution weight of CPDE can be tuned by different elliptical states of the excitation light. The photon-helicity-dependent THz emission from VGG based on CPDE offers an alternative thought of graphene-based polarization sensitive THz sources for chiral analysis in the THz field.
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