Rice U. lab finds evidence of matter-matter coupling

MIKE WILLIAMS
http://news.rice.edu/2018/08/23/rice-u-lab-finds-evidence-of-matter-matter-coupling/

HOUSTON – (Aug. 23, 2018) – After their recent pioneering experiments to couple light and matter to an extreme degree, Rice University scientists decided to look for a similar effect in matter alone. They didn’t expect to find it so soon.

Rice physicist Junichiro Kono, graduate student Xinwei Li and their international colleagues have discovered the first example of Dicke cooperativity in a matter-matter system, a result reported in Science this week.

Rice University scientists observed Dicke cooperativity in a magnetic crystal in which two types of spins, in iron (blue arrows) and erbium (red arrows), interacted with each other. The iron spins were excited to form a wave-like object called a spin wave; the erbium spins precessing in a magnetic field (B) behaved like two-level atoms. Illustration by Xinwei Li

The discovery could help advance the understanding of spintronics and quantum magnetism, Kono said. On the spintronics side, he said the work will lead to faster information processing with lower power consumption and will contribute to the development of spin-based quantum computing. The team’s findings on quantum magnetism will lead to a deeper understanding of the phases of matter induced by many-body interactions at the atomic scale.

Instead of using light to trigger interactions in a quantum well, a system that produced new evidence of ultrastrong light-matter coupling earlier this year, the Kono lab at Rice used a magnetic field to prompt cooperativity among the spins within a crystalline compound made primarily of iron and erbium.

“This is an emerging subject in condensed matter physics,” Kono said. “There’s a long history in atomic and molecular physics of looking for the phenomenon of ultrastrong cooperative coupling. In our case, we’d already found a way to make light and condensed matter interact and hybridize, but what we’re reporting here is more exotic.”

Dicke cooperativity, named for physicist Robert Dicke, happens when incoming radiation causes a collection of atomic dipoles to couple, like gears in a motor that don’t actually touch. Dicke’s early work set the stage for the invention of lasers, the discovery of cosmic background radiation in the universe and the development of lock-in amplifiers used by scientists and engineers.
                                              

Xinwei Li, left, and Junichiro Kono of Rice University led an international effort to find the first instance of Dicke cooperativity in a matter-matter system. Photo by Jeff Fitlow

“Dicke was an unusually productive physicist,” Kono said. “He had many high-impact papers and accomplishments in almost all areas of physics. The particular Dicke phenomenon that’s relevant to our work is related to superradiance, which he introduced in 1954. The idea is that if you have a collection of atoms, or spins, they can work together in light-matter interaction to make spontaneous emission coherent. This was a very strange idea.

“When you stimulate many atoms within a small volume, one atom produces a photon that immediately interacts with another atom in the excited state,” Kono said. “That atom produces another photon. Now you have coherent superposition of two photons.

“This happens between every pair of atoms within the volume and produces macroscopic polarization that eventually leads to a burst of coherent light called superradiance,” he said.

Taking light out of the equation meant the Kono lab had to find another way to excite the material’s dipoles, the compass-like magnetic force inherent in every atom, and prompt them to align. Because the lab is uniquely equipped for such experiments, when the test material showed up, Kono and Li were ready.

“The sample was provided by my colleague (and co-author) Shixun Cao at Shanghai University,” Kono said. Characterization tests with a small or no magnetic field performed by another co-author, Dmitry Turchinovich of the University of Duisburg-Essen, drew little response.

“But Dmitry is a good friend, and he knows we have a special experimental setup that combines terahertz spectroscopy, low temperatures and high magnetic field,” Kono said. “He was curious to know what would happen if we did the measurements.”

“Because we have some experience in this field, we got our initial data, identified some interesting details in it and thought there was something more we could explore in depth,” Li added.

“But we certainly didn’t predict this,” Kono said.

Li said that to show cooperativity, the magnetic components of the compound had to mimic the two essential ingredients in a standard light-atom coupling system where Dicke cooperativity was originally proposed: one a species of spins that can be excited into a wave-like object that simulates the light wave, and another with quantum energy levels that would shift with the applied magnetic field and simulate the atoms.

“Within a single orthoferrite compound, on one side the iron ions can be triggered to form a spin wave at a particular frequency,” Li said. “On the other side, we used the electron paramagnetic resonance of the erbium ions, which forms a two-level quantum structure that interacts with the spin wave.”

While the lab’s powerful magnet tuned the energy levels of the erbium ions, as detected by the terahertz spectroscope, it did not initially show strong interactions with the iron spin wave at room temperature. But the interactions started to appear at lower temperatures, seen in a spectroscopic measurement of coupling strength known as vacuum Rabi splitting.

Chemically doping the erbium with yttrium brought it in line with the observation and showed Dicke cooperativity in the magnetic interactions. “The way the coupling strength increased matches in an excellent manner with Dicke’s early predictions,” Li said. “But here, light is out of the picture and the coupling is matter-matter in nature.”

“The interaction we’re talking about is really atomistic,” Kono said. “We show two types of spin interacting in a single material. That’s a quantum mechanical interaction, rather than the classical mechanics we see in light-matter coupling. This opens new possibilities for not only understanding but also controlling and predicting novel phases of condensed matter.”

Co-authors of the paper are Motoaki Bamba, an associate professor at Osaka University; graduate students Ning Yuan, Maolin Xiang and Kai Xu and professors Zuanming Jin, Wei Ren and Guohong Ma at Shanghai University; Rice alumnus Qi Zhang, a research fellow at Argonne National Laboratory; and Yage Zhao, an undergraduate student at Peking University and former exchange student at Rice. Kono is a professor of electrical and computer engineering, of physics and astronomy, and of materials science and nanoengineering.

The research was supported by the National Science Foundation, the Army Research Office, the PRESTO program of the Japan Science and Technology Agency, the Japan Society for the Promotion of Science’s KAKENHI program, the ImPACT Program of the Government of Japan’s Council for Science, Technology and Innovation, the National Natural Science Foundation of China, German Research Foundation,the European Commission and the Max Planck Society.

Read the abstract at http://dx.doi.org/10.1126/science.aat5162

OT-Rice-sized laser, powered one electron at a time, bodes well for quantum computing

Princeton University researchers have built a rice grain-sized microwave laser. Credit: Jason Petta, Princeton University

http://phys.org/news/2015-01-rice-sized-laser-powered-electron-bodes.html#jCp

Princeton University researchers have built a rice grain-sized laser powered by single electrons tunneling through artificial atoms known as quantum dots. The tiny microwave laser, or "maser," is a demonstration of the fundamental interactions between light and moving electrons.

The researchers built the device—which uses about one-billionth the electric current needed to power a hair dryer—while exploring how to use quantum dots, which are bits of semiconductor material that act like single atoms, as components for quantum computers.

"It is basically as small as you can go with these single-electron devices," said Jason Petta, an associate professor of physics at Princeton who led the study, which was published in the journal Science.

The device demonstrates a major step forward for efforts to build quantum-computing systems out of semiconductor materials, according to co-author and collaborator Jacob Taylor, an adjunct assistant professor at the Joint Quantum Institute, University of Maryland-National Institute of Standards and Technology. "I consider this to be a really important result for our long-term goal, which is entanglement between quantum bits in semiconductor-based devices," Taylor said.

The original aim of the project was not to build a maser, but to explore how to use double quantum dots—which are two quantum dots joined together—as quantum bits, or qubits, the basic units of information in quantum computers.

"The goal was to get the double quantum dots to communicate with each other," said Yinyu Liu, a physics graduate student in Petta's lab. The team also included graduate student Jiri Stehlik and associate research scholar Christopher Eichler in Princeton's Department of Physics, as well as postdoctoral researcher Michael Gullans of the Joint Quantum Institute.

Double quantum dot as imaged by a scanning electron microscope. Current flows one electron at a time through two quantum dots (red circles) that are formed in an indium arsenide nanowire. Credit: Science

Because quantum dots can communicate through the entanglement of light particles, or photons, the researchers designed dots that emit photons when single electrons leap from a higher energy level to a lower energy level to cross the double dot.

Each double quantum dot can only transfer one electron at a time, Petta explained. "It is like a line of people crossing a wide stream by leaping onto a rock so small that it can only hold one person," he said. "They are forced to cross the stream one at a time. These double quantum dots are zero-dimensional as far as the electrons are concerned—they are trapped in all three spatial dimensions."

The researchers fabricated the double quantum dots from extremely thin nanowires (about 50 nanometers, or a billionth of a meter, in diameter) made of a semiconductor material called indium arsenide. They patterned the indium arsenide wires over other even smaller metal wires that act as gate electrodes, which control the energy levels in the dots.

To construct the maser, they placed the two double dots about 6 millimeters apart in a cavity made of a superconducting material, niobium, which requires a temperature near absolute zero, around minus 459 degrees Fahrenheit. "This is the first time that the team at Princeton has demonstrated that there is a connection between two double quantum dots separated by nearly a centimeter, a substantial distance," Taylor said.

When the device was switched on, electrons flowed single-file through each double quantum dot, causing them to emit photons in the microwave region of the spectrum. These photons then bounced off mirrors at each end of the cavity to build into a coherent beam of microwave light.

One advantage of the new maser is that the energy levels inside the dots can be fine-tuned to produce light at other frequencies, which cannot be done with other semiconductor lasers in which the frequency is fixed during manufacturing, Petta said. The larger the energy difference between the two levels, the higher the frequency of light emitted.

Claire Gmachl, who was not involved in the research and is Princeton's Eugene Higgins Professor of Electrical Engineering and a pioneer in the field of semiconductor lasers, said that because lasers, masers and other forms of coherent light sources are used in communications, sensing, medicine and many other aspects of modern life, the study is an important one.

"In this paper the researchers dig down deep into the fundamental interaction between light and the moving electron," Gmachl said. "The double quantum dot allows them full control over the motion of even a single electron, and in return they show how the coherent microwave field is created and amplified. Learning to control these fundamental light-matter interaction processes will help in the future development of light sources."

 Explore further: Arrays of electrons trapped in nanoscale circuitry could form the basis for future scalable quantum computers

More information: The paper, "Semiconductor double quantum dot micromaser," was published in the journal Science on Jan. 16, 2015. www.sciencemag.org/lookup/doi/… 1126/science.aaa2501

Journal reference: Science  

Provided by Princeton University  

Abstract-Toward Quantum Processing in Molecules: A THz-Bandwidth Coherent Memory for Light

Philip J. Bustard, Rune Lausten, Duncan G. England, and Benjamin J. Sussman^* 
National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6, Canada

http://prl.aps.org/abstract/PRL/v111/i8/e083901

The unusual features of quantum mechanics are enabling the development of technologies not possible with classical physics. These devices utilize nonclassical phenomena in the states of atoms, ions, and solid-state media as the basis for many prototypes. Here we investigate molecular states as a distinct alternative. We demonstrate a memory for light based on storing photons in the vibrations of hydrogen molecules. The THz-bandwidth molecular memory is used to store 100-fs pulses for durations up to ∼1  ns, enabling ∼10⁴ operational time bins. The results demonstrate the promise of molecules for constructing compact ultrafast quantum photonic technologies.

Work performed at the Institute of Terahertz Science and Technology Dept.UC Santa Barbara lead to a breakthrough in quantum computing

                                             (Credit: HZB/Radu)

Researchers develop quantum a computing system that resists 'quantum bug'

http://www.eurekalert.org/pub_releases/2011-07/uosc-ebu071811.php

Scientists have taken the next major step toward quantum computing, which will use quantum mechanics to revolutionize the way information is processed.

Quantum computers will capitalize on the mind-bending properties of quantum particles to perform complex calculations that are impossible for today's traditional computers.

Using high magnetic fields, Susumu Takahashi, assistant professor in the USC Dornsife College of Letters, Arts and Sciences, and his colleagues managed to suppress decoherence, which is one of the key stumbling blocks in quantum computing.

"High magnetic fields reduce the level of the noises in the surroundings, so they can constrain the decoherence very efficiently," Takahashi said. Decoherence has been described as a "quantum bug" that destroys fundamental properties that quantum computers would rely on.

This research will appear in the online version of Nature magazine on June 20.

Quantum computing uses quantum bits, or qubits, to encode information in the form of ones and zeros. Unlike a traditional computer that uses traditional bits, a quantum computer takes advantage of the fact seemingly impossible fact that qubits can exist in multiple states at the same time, which is called "superposition."

While can a bit can represent either a one or a zero, a qubit can represent a one and a zero at the same time due to superposition. This allows for simultaneous processing of calculations in a truly parallel system, skyrocketing computing ability.

Though the concepts underpinning quantum computing are not new, problems such as decoherence have hindered the construction of a fully functioning quantum computer.

Think of decoherence as a form of noise or interference, knocking a quantum particle out of superposition — robbing it of that special property that makes it so useful. If a quantum computer relies on a quantum particle's ability to be both here and there, then decoherence is the frustrating phenomenon that causes a quantum particle to be either here or there.

The researchers calculated all sources of decoherence in his experiment as a function of temperature, magnetic field, and by nuclear isotopic concentrations, and suggested the optimum condition to operate qubits, reducing decoherence by approximately 1,000 times.

Qubits in his experiment lasted about 500 microseconds at the optimum condition — ages, relatively speaking.

Decoherence in qubit systems falls into two general categories. One is an intrinsic decoherence caused by constituents in the qubit system, and the other is an extrinsic decoherence caused by imperfections of the system, for example, impurities and defects.

In their study, Takahashi and his colleagues investigated single crystals of molecular magnets. Because of their purity, molecular eliminate the extrinsic decoherence, allowing researchers to calculate intrinsic decoherence precisely.

"For the first time we've been able to predict and control all the environmental decoherence mechanisms in a very complex system — in this case a large magnetic molecule," said Phil Stamp, UBC professor of physics and astronomy and director of the Pacific Institute of Theoretical Physics.

Using crystalline molecular magnets allowed researchers to build qubits out of multiple quantum particles, rather than a single quantum object – the way most proto-quantum computers are built at the moment.

"This will obviously increase signals from the qubit drastically, so the detection of the qubit in the molecular magnets is much easier," Takahashi said.

Takahashi conducted his research as a project scientist in the Institute of Terahertz Science and Technology and Department of Physics at the University of California Santa Barbara and analyzed the data while at UCSB and USC. Takahashi has been in the USC Dornsife College since 2010.

Research for the article was performed in collaboration with Phil Stamp and Igor Tupitsyn of the University of British Columbia, Johan van Tol of Florida State University, and David Hendrickson of UC San Diego.

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This work was supported by the National Science Foundation, the W. M. Keck Foundation, the Pacific Institute of Theoretical Physics at UBC, by the Natural Sciences and Engineering Research Council of Canada, the Canadian Institute for Advanced Research and the USC startup funds.