Abstract-Ultrafast response of harmonic modelocked THz lasers

Feihu Wang, Valentino Pistore, Michael Riesch, Hanond Nong, Pierre-Baptiste Vigneron, Raffaele Colombelli, Olivier Parillaud, Juliette Mangeney, Jerome Tignon, Christian Jirauschek ,  Sukhdeep S. Dhillon

Fundamental and harmonic modelocking in the a time and b frequency domains

https://www.nature.com/articles/s41377-020-0288-x

The use of fundamental mode locking to generate short terahertz (THz) pulses and THz frequency combs from semiconductor lasers has become a routine affair, using quantum cascade lasers (QCLs) as a gain medium. However, unlike classic laser diodes, no demonstrations of harmonic modelocking, active or passive, have been shown in THz QCLs, where multiple pulses per round trip are generated when the laser is modulated at the harmonics of the cavity’s fundamental round-trip frequency. Here, using time-resolved THz techniques, we show for the first time harmonic injection and mode-locking in which THz QCLs are modulated at the harmonics of the round-trip frequency. We demonstrate the generation of the harmonic electrical beatnote within a QCL, its injection locking to an active modulation and its direct translation to harmonic pulse generation using the unique ultrafast nature of our approach. Finally, we show indications of self-starting harmonic emission, i.e., without external modulation, where the QCL operates exclusively on a harmonic (up to its 15th harmonic) of the round-trip frequency. This behaviour is supported by time-resolved simulations of induced gain and loss in the system and shows the importance of the electronic, as well as photonic, nature of QCLs. These results open up the prospect of passive harmonic modelocking and THz pulse generation, as well as the generation of low-noise microwave generation in the hundreds of GHz region.

Abstract-Room temperature terahertz semiconductor frequency comb

Quanyong Lu, Feihu Wang, Donghai Wu, Steven Slivker,  Manijeh Razeghi,

https://www.nature.com/articles/s41467-019-10395-7

A terahertz (THz) frequency comb capable of high-resolution measurement will significantly advance THz technology application in spectroscopy, metrology and sensing. The recently developed cryogenic-cooled THz quantum cascade laser (QCL) comb has exhibited great potentials with high power and broadband spectrum. Here, we report a room temperature THz harmonic frequency comb in 2.2 to 3.3 THz based on difference-frequency generation from a mid-IR QCL. The THz comb is intracavity generated via down-converting a mid-IR comb with an integrated mid-IR single mode based on distributed-feedback grating without using external optical elements. The grating Bragg wavelength is largely detuned from the gain peak to suppress the grating dispersion and support the comb operation in the high gain spectral range. Multiheterodyne spectroscopy with multiple equally spaced lines by beating it with a reference Fabry-Pérot comb confirms the THz comb operation. This type of THz comb will find applications to room temperature chip-based THz spectroscopy.

Abstract-Generating ultrafast pulses of light from quantum cascade lasers

Feihu Wang, Kenneth Maussang, Souad Moumdji, Raffaele Colombelli, Joshua R. Freeman, Iman Kundu, Lianhe Li, Edmund H. Linfield, A. Giles Davies, Juliette Mangeney, Jérôme Tignon, and Sukhdeep S. Dhillon

https://www.osapublishing.org/optica/abstract.cfm?uri=optica-2-11-944

The generation of ultrashort pulses from quantum cascade lasers (QCLs) has proved to be challenging. It has been suggested that the ultrafast electron dynamics of these devices is the limiting factor for mode locking and, hence, pulse formation. Even so, the clear mode locking of terahertz (THz) QCLs has been demonstrated recently, but the exact mechanism for pulse generation is not fully understood. Here we demonstrate that the dominant factor necessary for active pulse generation is in fact the synchronization between the propagating electronic modulation and the generated THz pulse in the QCL. By using the phase-resolved detection of the electric field in QCLs embedded in metal–metal waveguides, we demonstrate that active mode locking requires the phase velocity of the microwave round-trip modulation to equal the group velocity of the THz pulse. This allows the THz pulse to propagate in phase with the microwave modulation along the gain medium, permitting short-pulse generation. Mode locking was performed on QCLs employing phonon depopulation active regions, permitting the coherent detection of large gain bandwidths (500 GHz) and the generation of 11 ps pulses centered around 2.6 THz when the above “phase-matching” condition is satisfied. This work brings an enhanced understanding of QCL mode locking and will permit new concepts to be explored to generate shorter and more intense pulses from mid-infrared, as well as THz, QCLs.

© 2015 Optical Society of America

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