Wednesday, May 13, 2020

IR Laser Mixing, Optical “Magic” Yields THz Waves with Relative Efficiency



By mixing and manipulating an infrared laser, a team led by researchers at TU Wein (Vienna University of Technology) has generated a wide band of terahertz waves with relatively high efficiency.

The terahertz segment of the electromagnetic spectrum exists in a sort of “twilight zone” between about 300 GHz (0.3 THz) to 3 THz (note that the upper boundary value is somewhat arbitrary, and some consider it to be 30 THz). It’s bounded below by millimeter-wave RF (30 to 300 GHz) and above by optical wavelengths. Electromagnetic radiation below the terahertz band can be created by many sources and emitted by antennas, while the optical radiation above the terahertz band can be developed by solid-state lasers.

However, the major part of the terahertz span is largely a void. Although it’s governed by Maxwell’s equations just as the rest of the spectrum, it’s relatively difficult to generate these waves as they’re too high in frequency for even most leading-edge electronic components and too low for optical sourcing. Due to this and other problems, the terahertz region is far less explored and exploited than the RF or optical areas (see “References” at end of article).
Why even investigate the terahertz part of the spectrum? Among the many reasons are because it’s there, of course; because it potentially has useful and fascinating characteristics; and it may be needed for 6G, 7G, or 8G wireless links. After all, 20 years ago, if you had told someone that there would be mass-market consumer products operating at ~10 GHz by the first part of the 21st century, you would have likely been called a wild-eyed dreamer.
Power Problems
However, the problem remains in terms of efficiently generating useful levels of power in the terahertz band. There are tabletop sources based on either optical rectification in electro-optic crystals or two-color filamentation in gases and liquids. With optical rectification, terahertz pulses with energy up to 0.9 mJ and THz conversion efficiency (ratio of generated THz energy to the input laser pulse energy) up to 3.7% have been generated, but the pulses are long (several picoseconds) with narrow spectra.
Unfortunately, the optical-damage threshold of electro-optic crystals prevents a significant increase in power. Furthermore, while there are no issues with optical damage when using the two-color filamentation approach, it generates only less-energetic near-infrared (NIR) laser pulses, and with a very low conversion efficiency of ~0.01%.
Efficient Source Breakthrough
Now, a research group based at TU Wein (Vienna University of Technology), in close cooperation with a team from the Institute of Electronic Structure and Laser (IESL) Foundation for Research and Technology-Hellas (FORTH) in Heraklion, Greece, and some help from Texas A&M University at Qatar, has developed a source that’s both fairly efficient and can generate waves across the entire terahertz slice of spectrum. The experiment, with results they claim has broken previous records in these areas, was inspired by a theory developed in Texas A&M University, which predicted that long-wavelength laser pulses could be used to achieve extremely efficient terahertz generation in air plasma.
In the setup schematic (Fig. 1), the generation of the terahertz waves begins by sending infrared laser light through a nonlinear medium, where part of the infrared radiation is transformed into optical radiation at twice the initial frequency. The two radiation waves are then superimposed, creating an electromagnetic wave with an electric field having a very specific asymmetric shape.
The setup for THz generation by two-color mid-infrared filaments (a). After the quarter wave plate (QWP), the 3.9-μm laser pulse passes through the gallium-selenide (GaSe) crystal and generates the second harmonic pulse. The two-color laser pulse is focused by an off-axis parabolic mirror (OPM1) in ambient air and forms a filament where the THz radiation is generated. A parabolic mirror (OPM2) gathers the emitted THz pulse and guides it into one of the detection setups. The metallic disk (MD) blocks the on-axis mid-infrared radiation and generated supercontinuum, while the conically emitted THz radiation passes around it. A set of lowpass filters filter out the remained unwanted radiation and prevent the saturation of the pyroelectric detector (PED) by the intense THz pulses. THz detection setups (b-d): The parabolic mirror (OPM3) focuses the THz pulse on the PED to measure its energy (b). The wire grid polarizer (GP), placed before the OPM3, makes it possible to characterize the THz polarization. For the electro-optic measurements, the parabolic mirror (OPM4) focuses the THz pulse into a 55-μm thick gallium phosphide (GaP) crystal (c). A pair of GPs reduces the THz field strength to ensure a linear response. The 680-nm synchronized probe pulse focuses into the GaP crystal through a hole in OPM4 and then is guided to the balanced detection setup. For the cross-phase modulation experiment, the GaP crystal is replaced by the 1-mm-thick zinc-telluride (ZnTe) crystal and the 761-nm probe pulse is guided to the spectrometer. The Michelson interferometer measures the THz field autocorrelation and consists of a pellicle beam splitter (PBS) and two flat mirrors: fixed (M1) and movable (M2) (d). At the exit, a parabolic mirror (OPM5) focuses the radiation on the PED. (Source: TU Wein)

But that’s only the start of this process. The intense wave “rips” electrons out of the molecules in the air, turning the air into a glowing plasma. The special shape of the wave's electric field accelerates the electrons in such a way that they produce the desired terahertz radiation.
As noted by team member Claudia Gollner (Fig. 2), “Our method is extremely efficient with 2.3% of the supplied energy converted into terahertz radiation. That is orders of magnitude more than can be achieved with other methods. This results in exceptionally high terahertz energies of almost 200 microjoules and terahertz-field amplitudes exceeding 100 MV per cm.”
Researcher Claudia Gollner adjusts the optoelectronic setup in the lab at TU Wein’s photonics institute. (Source: TU Wein)
She also added that their approach develops many wavelengths throughout the terahertz range to be emitted simultaneously, and the larger spectrum of different terahertz wavelengths yields the shorter and more intense pulses.
The details, including a review of existing methods of terahertz generation and their characteristics, are in their paper “Observation of extremely efficient terahertz generation from mid-infrared two-color laser filaments” published in Nature Communications, along with even-more detailed, equation-laced Supplementary Information.
References
IEEE Spectrum, “The Truth About Terahertz

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