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The characteristics of terahertz (THz) modulation in organic copper phthalocyanine thin films deposited on a Si wafer were investigated by angle-dependent photoexcitation. We reveal that the efficiency of THz modulation reflects not only the angle-dependent reflectivity of the organic thin films that undergo a change of complex refractive index due to photoexcitation but also the laser-induced birefringence induced by a charge density grating in the direction normal to the polarization of the excitation beams.
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