The hot debate regarding attosecond dynamics of optical tunneling has, so far, been focused on the presence, or absence, of time delays associated to the electron tunnelling through the classically forbidden region during atomic ionization in intense infrared laser fields. Strong theoretical and experimental arguments have been put forward to advocate the polar opposite points of view. The underlying dynamics are richer. Here we propose to use the nonlinear optical responses of the tunnelling electrons to tailored light fields to track these dynamics in full complexity. Using the combination of single-color and two-color fields, we resolve not only ionization delays, but also temporal re-shaping and spatial re-focusing of the tunnelling wavepacket as it emerges from the classically forbidden region. Access to these details of the dynamics is facilitated by the near-instantaneous nature of the nonlinear optical response driven by ionization, and by using tailored laser pulses to induce this response. Our work introduces a new type of attoclock for optical tunnelling, one that is based on measuring light rather than photo-electrons. Our conclusions suggest a possible middle ground between the two conflicting points of view.
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Showing posts with label M. Ivanov. Show all posts
Showing posts with label M. Ivanov. Show all posts
Friday, March 23, 2018
Abstract-All-optical attoclock: accessing exahertz dynamics of optical tunnelling through terahertz emission
Thursday, December 21, 2017
Abstract-Symmetry Breaking and Strong Persistent Plasma Currents via Resonant Destabilization of Atoms
C. Brée, M. Hofmann, A. Demircan, U. Morgner, O. Kosareva, A. Savel’ev, A. Husakou, M. Ivanov, and I. Babushkin
The ionization rate of an atom in a strong optical field can be resonantly enhanced by the presence of long-living atomic levels (so-called Freeman resonances). This process is most prominent in the multiphoton ionization regime, meaning that the ionization event takes many optical cycles. Nevertheless, here, we show that these resonances can lead to rapid subcycle-scale plasma buildup at the resonant values of the intensity in the pump pulse. The fast buildup can break the cycle-to-cycle symmetry of the ionization process, resulting in the generation of persistent macroscopic plasma currents which remain after the end of the pulse. This, in turn, gives rise to a broadband radiation of unusual spectral structure, forming a comb from terahertz to visible. This radiation contains fingerprints of the attosecond electron dynamics in Rydberg states during ionization.
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