Speaker: Mengkun Liu, UC-San Diego
Thursday, January 30th 2014 -
ABSTRACT: In strongly correlated electron materials (CEMs), the delicate interplay between spin, charge, and lattice degrees of freedom often leads to extremely rich phase diagrams exhibiting intrinsic phase inhomogeneities. The key to studying and disentangling such complexities usually lies in characterization and control of these materials at their fundamental energy, time and length scales. Using the prototypical correlated insulator vanadium dioxide (VO2) as a case study, I will show in this talk that ultrafast and ultrasmall optical spectroscopy offers unique insights into this electronic/structural interplay with unprecedented spatial and temporal resolutions. Specifically, with scanning near-field infrared microscopy we resolved the long-lasting enigma of electronic anisotropy in VO2 and revealed three distinct stages of the insulator to metal transition (IMT) at nanoscopic length scales. Using ultrafast terahertz pump terahertz probe spectroscopy we have also unambiguously demonstrated that the IMT occurs at picosecond time scales via electric field-induced electron liberation. These results set the stage for future spectroscopic investigations to access the fundamental time and length scales of CEMs.
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