Abstract-Flexible and giant terahertz modulation based on ultra strain sensitive conductive polymer composites

Qiwu Shi, Ke Tian, Hongfu Zhu, Zi-run Li, Li-Guo,  Zhu Hua,  Deng Wanxia Huang, Qiang Fu,

https://pubs.acs.org/doi/10.1021/acsami.9b21890

Dynamic tuning of terahertz (THz) wave has a great potential application for smart THz devices, such as switching, modulation, sensor, and so on. However, realization of flexible THz modulation with high efficiency is rarely observed, which is nearly absent from the booming development and demands on flexible electronics. Here, we report a flexible THz modulation based on conductive polymer composites composed of thermoplastic polyurethane (TPU) and conductive particles (Ni). By designing the additive content of Ni particles, such flexible layer exhibits resistivity change of 6-7 orders under tensile strain, due to the formation of electron transport channel provided by in situ evolution of Ni network. It could be used to dynamically control THz transmission with giant modulation depth of around 96%, at high strain operation (up to around 58.5%). Moreover, these characteristics are demonstrated to be available for highly tension sensitive THz spectroscopy and imaging. This work opens up a connection between flexible polymer based composites and THz dynamic device. It proposes an unprecedented flexible THz modulation with giant tuning efficiency, and provides a scheme for contactless and passive tension sensor.

Abstract-Dynamic Photoinduced Controlling of the Large Phase Shift of Terahertz Waves via Vanadium Dioxide Coupling Nanostructures

Yuncheng Zhao, Yaxin Zhang, Qiwu Shi, Shixiong Liang,  Wanxia Huang,  Wei Kou,  Ziqiang Yang,

https://pubs.acs.org/doi/10.1021/acsphotonics.8b00276

Utilizing terahertz (THz) waves to transmit data for communication and imaging places high demands on phase modulation. However, until now, it is difficult to realize a more than 100° phase shift in the transmission mode with one-layer structure. In this paper, a ring-dumbbell composite resonator nested with VO2 nanostructures is proposed to achieve the large phase shift. It is found that in this structure a hybrid mode with an enhanced resonant intensity, which is coupled by the L-C resonance and dipole resonance has been observed. Applying the photoinduced phase transition characteristics of VO2, the resonant intensity of the mode can be dynamically controlled, which leads to a large phase shift in the incident THz wave. The dynamic experimental results show that controlling the power of the external laser can achieve a phase shift of up to 138° near 0.6 THz using this one-layer VO2 nested composite structure. Moreover, within a 55 GHz (575–630 GHz) bandwidth, the phase shift exceeds 130°. This attractive phase shift modulation may provide prospective applications in THz imaging, communications, and so on.

Abstract-Dynamic Photo-induced Controlling of the Large Phase Shift of Terahertz Waves via Vanadium Dioxide Coupling Nanostructures

Yuncheng Zhao, Yaxin Zhang, Qiwu Shi, Shixiong Liang, Wanxia Huang, Wei Kou, Ziqiang Yang,

https://pubs.acs.org/doi/abs/10.1021/acsphotonics.8b00276?mi=aayia761&af=R&AllField=nano&target=default&targetTab=std

Utilizing terahertz (THz) waves to transmit data for communication and imaging places high demands on phase modulation. However, until now, realizing a large phase shift using a one-layer structure in transmission mode has been difficult. In this paper, utilizing a composite unit cell by coupling the traditional metallic wire dipolar resonance and the split-ring capacitive inductance resonance results in an enhanced resonance coupling mode. Combined with a vanadium dioxide (VO2) nanostructure and applying the photo-induced phase transition, the resonant intensity of the mode can be dynamically controlled, which leads to an ultralarge phase shift in the incident THz wave. The dynamic experimental results show that controlling the power of the external laser can achieve a phase shift of up to 138 degrees near 0.6 THz using this one-layer VO2 nested composite structure. Moreover, within a 55 GHz (575 GHz-630 GHz) bandwidth, the phase shift exceeds 130 degrees. This attractive phase shift modulation may provide prospective applications in THz imaging, communications, etc.