Showing posts with label Max Planck Research Department for Structural Dynamics (MPSD). Show all posts
Showing posts with label Max Planck Research Department for Structural Dynamics (MPSD). Show all posts

Wednesday, April 3, 2013

Light tsunami in a superconductor




An international team of researchers investigated light tsunamis in a superconductor using the HZDR free electron laser's strong terahertz flashes. Credit: Frank Bierstedt
: http://phys.org/news/2013-04-tsunami-superconductor.html#jCp
Superconductors are materials which conduct electric currents without any resistance. At the Helmholtz-Zentrum Dresden-Rossendorf, an international research team headed by Professor Andrea Cavalleri from the Max Planck Institute for the Structure and Dynamics of Matter managed to selectively influence this resistance-free conductivity with a powerful terahertz laser. This very precise laser light turns into a vortex which moves through the superconductor like a tsunami. The results will be published in the scientific journal Nature Materials


In their latest experiment, Prof. Andrea Cavalleri from the Max Planck Institute for the Structure and Dynamics of Matter at the Hamburg-based Center for Free-Electron Laser Science (CFEL) and Dr. Michael Gensch from the Helmholtz-Zentrum Dresden-Rossendorf (HZDR) investigated together with other colleagues from the HZDR, the United Kingdom, and Japan if and how superconductivity can be systematically controlled. The objective of their research is to improve the usability of superconducting materials for such new technologies as, for example, the processing of information. For this purpose, and for a better understanding of the underlying phenomena, it is essential to increase the critical temperature – critical temperature means that materials below this value are superconducting. Today, most superconductors only function at very low temperatures.

Typically, modern high temperature superconductors are solids which consist of a stack of thin layers, similar to the pages in a book. These layers are conductive and transport electricity. However, no electricity can flow from layer to layer at room temperature since those electrons which are responsible for the current flow can only move freely in the respective layer. If, however, such a layer stack is cooled to the right temperature, then superconductivity occurs along all directions. But there is one difference: While the electrons flow inside a layer without any resistance, these electrons can now also move from layer to layer by "tunneling" through the insulating areas located between these layers. Dr. Gensch explains: "Already the geometry suggests that the mechanisms of superconductivity are different inside and between the layers. We were interested in how the electrons transport this property vertically from layer to layer and/or whether we would be able to control this transport without disrupting the superconductivity in the horizontal layers."


For their experiments, the researchers used one of the HZDR's two free electron lasers (FELBE) which generates laser flashes of a specific, freely adjustable wavelength between the infrared and the microwave range. If such a short terahertz flash penetrates the material layers of the superconductor at the right frequency, then it deactivates the superconductivity very selectively and locally by directly changing the tunneling properties of the electrons found between the superconducting layers. More precisely, the light generates a pair of normal-conducting vortex currents which rotate in opposite directions. These vortices then move through the superconductor with the light. A so-called soliton wave is formed. What's so special about these waves: They always retain their shape irrespective of any faults in the superconductor. This resembles the behavior of such known soliton waves as, for example, tsunamis; the shape of which is also not influenced by any ground dislocations or irregularities
The vortices moving through the superconductor also alter the optical properties of the material – it becomes slightly transparent. While not for visible light, this is the case for wavelengths in the terahertz regime. The laser flashes last only for a few picoseconds, i.e. the billionth part of a second, so the scientists are able to observe all processes – such as the emergence of the vortices and their soliton movement – directly along this very fast time scale. The team headed by Prof. Cavalleri had successfully achieved something similar already once before. But back then, the scientists had only been able to quickly and consecutively switch the entire superconductivity off and on again between the layers. For the first time ever, the experiment in Dresden successfully managed to switch off the superconductivity very precisely and, above all, also locally – and to stabilize this state almost ten times longer than has been the case before.


In particular, the physicists expect a number of new applications from these light generated vortices inside superconductors. Since they move through the crystal just like a tsunami irrespective of any faults or irregularities, these vortices are perfectly suited to store and transport information inside them. Information is transported within DNA like soliton waves. The experiment, which furnished proof and demonstrated that the vortices can be controlled by laser light, has the physicists in Prof. Cavalleri's team already dreaming about new opportunities for information processing in superconductors.

Superconductors under Constant Bombardment


For a number of years now, intense pulses in the invisible terahertz range (0.1 THz – 10 THz) have been sparking enormous interest among scientists who investigate such so-called complex materials as high temperature superconductors. This is due to the specific properties of this long-wave radiation which has wavelengths between 0.03 and three millimeters. The energy per light particle is so low that the radiation doesn't really interact anymore directly with the electrons in a material, but instead, for example, with the atomic lattice. Sufficiently strong sources have been available for this purpose only for a couple of years now. The strongest terahertz pulses are generated by devices which are powered by electron accelerators.


The HZDR is specialized in a particularly important type of source for material sciences at the Center for High-Performance Radiation Sources called ELBE. While other devices have to take a break after a small series of ultrashort laser flashes, the ELBE sources are able to maintain a constant bombardment. It is actually this continuous sequence of pulses which permits the accuracy that researchers like Dr. Gensch and their guest researchers, such as Prof. Cavalleri, need for their analyses. In order to cover the entire spectral range down to 0.1 terahertz and three millimeter wavelengths, respectively, with even more intense pulses in the future, the HZDR is establishing a new, superradiant terahertz source called TELBE under the supervision of Dr. Gensch. Superradiance means here that extremely intense light is produced in a novel avalanche-like, short process without needing any mirrors as resonators – unlike, for example, free electron lasers. This allows generating even higher terahertz fields at much more flexible repetition rates. Over the next three years, the new TELBE facility will be put into operation and commissioned with the assistance of selected pilot users. The researchers hope to utilize TELBE to unravel new phenomena in the field of materials research as well as life sciences.






Tuesday, November 20, 2012

Physicists demonstrate crucial method for monitoring ultra short X-ray pulses



A single-cycle terahertz field accelerates photoelectrons emitted from neon atoms irradiated by an X-ray free-electron laser. In this way, the X-ray pulse temporal profile and arrival time are uniquely retrieved on a pulse-to-pulse basis with femtosecond precision. Credit: Jörg Harms/MPSD at CFEL
Read more at: http://phys.org/news/2012-11-physicists-crucial-method-ultra-short.html#jCp
http://phys.org/news/2012-11-physicists-crucial-method-ultra-short.html#jCp
With their ultra short X-ray flashes, free-electron lasers offer the opportunity to film chemical reactions or atoms in motion. However, for this super slow motion the arrival time and the temporal profile of the pulses must be precisely known. An international team of scientists has now developed a measurement technique that provides complete temporal characterization of individual FEL (free-electron laser) pulses at DESY´s soft-X-ray free-electron laser FLASH. The team, led by Adrian Cavalieri from the Center for Free-Electron Laser Science (CFEL) in Hamburg, was able to measure the temporal profile of each X-ray pulse with femtosecond precision (a femtosecond is a quadrillionth of a second). Their technique can be implemented at any of the world´s X-ray free-electron lasers, ultimately allowing for most effective utilization of these sources. The results are published in the current issue of the scientific journal Nature Photonics.

X-ray pulses delivered by free-electron lasers provide unique research opportunities, because the pulses are ultra-intense and ultra-short. At FELs trillions of X-ray photons are packed within a single burst – or pulse – which lasts for only several tens of femtoseconds, or even less. However, the precise arrival time and even the temporal profile of the FEL pulse can change dramatically from one pulse to the next.Therefore, to use the FEL to "film" ultrafast dynamical processes, the arrival time of each pulse must be measured to reorder the individual frames or snapshots captured with each individual FEL pulse. Provided with accurate timing information, femtosecond FEL X-ray pulses are short enough to study atoms in motion, chemical reactions, and phase transitions in materials with atomic resolution on the femtosecond timescale. With simultaneous measurement of the FEL X-ray pulse profile, it will be possible to go even further, to explore processes that evolve within the X-ray exposure. On these timescales the motion of electrons and electronic state dynamics become significant. Electronic dynamics drive damage processes in biomolecules, which may destroy them before they can be recorded in a crystal clear image. For their measurements, the team which includes scientists from CFEL, DESY, European XFEL, University of Hamburg and SLAC adapted a technique used in attosecond science called "photoelectron streaking" (an attosecond is a thousandth of a femtosecond). With this, the temporal profiles of varying light signals can be recorded. By taking advantage of the ultra-high intensities available at FELs the researchers were able to perform the streaking measurement on a single-shot basis at FLASH. For this, the X-ray flashes were shot through neon gas on their way to their target. Each pulse ejects a burst of photoelectrons from the noble gas. The temporal profile of the photoelectrons is a replica of the FEL pulse that ejected them. With an electromagnetic terahertz (THz) field, the photoelectrons are accelerated or decelerated, depending on the exact instant of their ejection. The strength of this effect is measured using time-of-flight spectroscopy. If the exact shape of the terahertz pulse is known, combining this information reveals the temporal profile and arrival time of the individual X-ray pulses with a precision of about 5 femtoseconds. "Simultaneous measurement of the arrival time and pulse profile, independent of all other FEL parameters, is the key to this technique," explains Cavalieri, who is a professor at the University of Hamburg and a group leader in the Max Planck Research Department for Structural Dynamics (MPSD). Until now, no other measurement has provided this complete timing information – yet it is exactly this information that will be crucial for future application of these unique X-ray light sources. The FEL pulse characterization measurements presented by the team are made without affecting the FEL beam – only a negligible number of photons are lost for creating photoelectrons. Therefore, they can be applied in any experiment at almost any wavelength, for example at the European XFEL which is currently under construction in Northern Germany. In the immediate future, laser-driven THz streaking will be used to monitor and maintain the FEL pulse duration at FLASH to study a wide variety of atomic, molecular and solid-state systems. For further experiments, the researchers plan to use these high precision measurements as critical feedback for tailoring and manipulating the X-ray pulse profile.
 More information: Grguras, I. et al., Ultrafast X-ray pulse characterization at free-electron lasers.
Nature Photonics, 2012 (advance online publication);
DOI: 10.1038/NPHOTON.2012.276
Journal reference: Nature Photonics