http://www.nature.com/articles/srep21169
Terahertz quantum cascade laser sources based on intra-cavity difference-frequency generation are currently the only room-temperature mass-producible diode-laser-like emitters of coherent 1–6 THz radiation. Device performance has improved dramatically over the past few years to reach milliwatt-level power output and broad tuning from 1.2 to 5.9 THz, all at room-temperature. Terahertz output in these sources originates from intersubband optical nonlinearity in the laser active region. Here we report the first comprehensive spectroscopic study of the optical nonlinearity and investigate its dependence on the mid-infrared pump frequencies. Our work shows that the terahertz generation efficiency can vary by a factor of 2 or greater depending on the spectral position of the mid-infrared pumps for a fixed THz difference-frequency. We have also measured for the first time the linewidth for transitions between the lower quantum cascade laser states, which is critical for determining terahertz nonlinearity and predicting optical loss in quantum cascade laser waveguides.
Karun Vijayraghavan,, Yifan Jiang
, Min Jang ,
Aiting Jiang, Karthik Choutagunta, , Augustinas Vizbaras, Frederic Demmerle,, Gerhard Boehm
, Markus C. Amann, Mikhail A. Belkin
Room temperature, broadly tunable, electrically pumped semiconductor sources in the terahertz spectral range, similar in operation simplicity to diode lasers, are highly desired for applications. An emerging technology in this area are sources based on intracavity difference-frequency generation in dual-wavelength mid-infrared quantum cascade lasers. Here we report terahertz quantum cascade laser sources based on an optimized non-collinear Cherenkov difference-frequency generation scheme that demonstrates dramatic improvements in performance. Devices emitting at 4 THz display a mid-infrared-to-terahertz conversion efficiency in excess of 0.6 mW W−2 and provide nearly 0.12 mW of peak power output. Devices emitting at 2 and 3 THz fabricated on the same chip display 0.09 and 0.4 mW W−2 conversion efficiencies at room temperature, respectively. High terahertz-generation efficiency and relaxed phase-matching conditions offered by the Cherenkov scheme allowed us to demonstrate, for the first time, an external-cavity terahertz quantum cascade laser source tunable between 1.70 and 5.25 THz.
http://proceedings.spiedigitallibrary.org/proceeding.aspx?articleid=1380680
Karun Vijayraghavan ; Augustinas Vizbaras ; Robert W. Adams ; Min Jang ; Christian Grasse ; Gerhard Boehm ; Markus C. Amann ; Mikhail A. Belkin
Room-temperature terahertz (THz) quantum cascade laser (QCL) sources based on intra-cavity difference-frequency generation (DFG) with record THz conversion efficiencies is reported. THz DFG QCLs reported previously are highly inefficient since THz radiation produced more than ~100 μm away from the exit facet is fully absorbed due to high THz losses in the QCL waveguide. Our lasers use a non-collinear Čerenkov DFG scheme to extract THz radiation from the active region. Dual-color mid-infrared quantum cascade lasers with integrated giant optical nonlinearity are grown on semi-insulating (S.I.) InP substrates. A lateral current extraction scheme is used. THz radiation is emitted at an angle into the substrate with respect to the mid-infrared pumps. Since S.I. InP is virtually lossless to THz radiation, this scheme allows for efficient extraction of THz radiation along the whole waveguide length. As a result, our sources demonstrate large mid-infrared-to-THz conversion efficiency and directional THz output. Experimentally, proof-of-principle devices demonstrate a conversion efficiency up to 70 μW/W2 and provide output across a 1.2 - 4.5 THz spectral range.© (2012) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
