Showing posts with label JIang Li. Show all posts
Showing posts with label JIang Li. Show all posts

Sunday, February 14, 2021

Abstract-Optical Kerr nonlinearity and multi-photon absorption of DSTMS measured by Z-scan method

 

 https://arxiv.org/abs/2102.03242

We investigate the optical Kerr nonlinearity and multi-photon absorption (MPA) properties of DSTMS excited by femtosecond pulses at a wavelengths of 1.43 {\mu}m, which is optimal for terahertz generation via difference frequency mixing. The MPA and the optical Kerr coefficients of DSTMS at 1.43 {\mu}m are strongly anisotropic indicating a dominating contribution from cascaded 2nd-order nonlinearity. These results suggest that the saturation of the THz generation efficiency is mainly related to the MPA process and to a spectral broadening caused by cascaded 2nd-order frequency mixing within DSTMS

Saturday, December 12, 2020

Abstract-Near‐Field Nanoscopic Terahertz Imaging of Single Proteins

 


Zhongbo Yang,  Dongyun Tang,  Jiao Hu,  Mingjie Tang,  Mingkun Zhang,  Hong‐Liang, Cui  Lihua Wang,  Chao Chang,  Chunhai Fan,  Jiang Li,  Huabin Wang,



https://onlinelibrary.wiley.com/doi/abs/10.1002/smll.202005814

Terahertz (THz) biological imaging has attracted intense attention due to its capability of acquiring physicochemical information in a label‐free, noninvasive, and nonionizing manner. However, extending THz imaging to the single‐molecule level remains a challenge, partly due to the weak THz reflectivity of biomolecules with low dielectric constants. Here, the development of graphene‐mediated THz scattering‐type scanning near‐field optical microscope for direct imaging of single proteins is reported. Importantly, it is found that a graphene substrate with high THz reflectivity and atomic flatness can provide high THz contrast against the protein molecules. In addition, a platinum probe with an optimized shaft length is found enabling the enhancement of the amplitude of the scattered THz near‐field signals. By coupling these effects, the topographical and THz scattering images of individual immunoglobulin G (IgG) and ferritin molecules with the size of a few nanometers are obtained, simultaneously. The demonstrated strategy thus opens new routes to imaging single biomolecules with THz

Sunday, June 14, 2020

Abstract-Ghost spintronic THz-emitter-array microscope


Si-Chao Chen, Zheng Feng, Jiang Li, Wei Tan, Liang-Hui Du, Jianwang Cai, Yuncan Ma, Kang He, Haifeng Ding, Zhao-Hui Zhai, Ze-Ren Li, Cheng-Wei Qiu, Xi-Cheng Zhang,  Li-Guo Zhu


https://www.nature.com/articles/s41377-020-0338-4

Terahertz (THz) waves show great potential in nondestructive testing, biodetection and cancer imaging. Despite recent progress in THz wave near-field probes/apertures enabling raster scanning of an object’s surface, an efficient, nonscanning, noninvasive, deep subdiffraction imaging technique remains challenging. Here, we demonstrate THz near-field microscopy using a reconfigurable spintronic THz emitter array (STEA) based on the computational ghost imaging principle. By illuminating an object with the reconfigurable STEA followed by computing the correlation, we can reconstruct an image of the object with deep subdiffraction resolution. By applying an external magnetic field, in-line polarization rotation of the THz wave is realized, making the fused image contrast polarization-free. Time-of-flight (TOF) measurements of coherent THz pulses further enable objects at different distances or depths to be resolved. The demonstrated ghost spintronic THz-emitter-array microscope (GHOSTEAM) is a radically novel imaging tool for THz near-field imaging, opening paradigm-shifting opportunities for nonintrusive label-free bioimaging in a broadband frequency range from 0.1 to 30 THz (namely, 3.3–1000 cm−1).

Saturday, April 25, 2020

Abstract-Design of terahertz-wave Doppler interferometric velocimetry for detonation physics

Publisher Logo


Zhao-Hui Zhai, Chang-Lin Sun, Qiao Liu,, Liu-Wei Guo, Yu-Si Liu, Xu Zhang,  De-Tian Wang, Kun Meng, Jiang Li,  Liang-Hui Du,  Shou-Xian Liu, Sen-Cheng Zhong,  Li-Guo Zhu,

(a) Schematic diagram of the TDV system (dashed box) and the detonation testing field. See the supplementary material for the details. (b) THz transmission efficiency vs distance between L3 and L4, assuming the THz beam waist of the TDV output is 15 mm and L4 has a diameter of 50 mm (solid lines) or 30 mm (dashed lines). (c) Simulated THz beam diameter and field depth inside the target for various numerical apertures (NAs) of L4 (assuming n =1.7). The red circles in (b) and (c) are the parameters of the prototype PDV system.
https://aip.scitation.org/doi/abs/10.1063/1.5142415

The diagnosis of the initiation and growth of detonation in high explosives (HEs) is important in detonation physics. We designed and experimentally demonstrated a non-invasive high-precision free-space terahertz-wave Doppler interferometric velocimetry (TDV) design for diagnosing the transient detonation processes in HEs. The system can non-intrusively record the propagation of the shock/detonation wavefront inside HEs continuously and measure key detonation parameters (position/displacement, detonation velocity, etc.). A detailed quasi-optical design for TDV is discussed. The terahertz penetration ability and the refractive index of representative HEs are presented in the frequency range of 0.2–1.4 THz. Additionally, a typical shock-to-detonation transition of an insensitive high explosive was studied using a prototype 0.212 THz TDV system, which demonstrated the high precision of displacement measurements made using I/Q demodulation. Furthermore, the performance of the TDV technique is discussed. TDV may enable non-invasive and high-precision diagnostics for detonation and shockwave physics.
The National Science Foundation of China (Grant Nos. 61427814, 11704358, and 11604316) and the Foundation of CAEP (Grant No. CX20200001).
The authors own related patents (Nos. CN105807082B, CN105509817B, and CN108398691A).
The authors would like to thank Z. Q. Liu, J. H. Meng, J. H. Tian, P. Gao, and L. H. He for their help with the detonation experiments.

Saturday, March 14, 2020

Abstract-Single cell imaging with near‐field terahertz scanning microscopy



Zaoxia Li, Shihan Yan, Ziyi Zang, Guoshuai Geng, Zhongbo Yang, Jiang Li, Lihua Wang, Chunyan Yao, Hong‐Liang Cui, Chao Chang, Huabin Wang


https://onlinelibrary.wiley.com/doi/full/10.1111/cpr.12788

Objectives

Terahertz (THz)‐based imaging techniques hold great potential for biological and biomedical applications, which nevertheless are hampered by the low spatial resolution of conventional THz imaging systems. In this work, we report a high‐performance photoconductive antenna microprobe‐based near‐field THz time‐domain spectroscopy scanning microscope.

Materials and methods

A single watermelon pulp cell was prepared on a clean quartz slide and covered by a thin polyethylene film. The high performance near‐field THz microscope was developed based on a coherent THz time‐domain spectroscopy system coupled with a photoconductive antenna microprobe. The sample was imaged in transmission mode.

Results

We demonstrate the direct imaging of the morphology of single watermelon pulp cells in the natural dehydration process with our near‐field THz microscope.

Conclusions

Given the label‐free and non‐destructive nature of THz detection techniques, our near‐field microscopy‐based single‐cell imaging approach sheds new light on studying biological samples with THz.


Tuesday, April 23, 2019

Abstract-A near-perfect THz modulator enabled by impedance matching method with VO2thin films



Liang-Hui Du, Hong-Fu Zhu,  Jiang Li, Qi-Wu Shi,  Li-Guo Zhu

https://ieeexplore.ieee.org/document/8510388

We present a terahertz (THz) amplitude modulator with near perfect modulation depth based on the impedance matching method during the thermally induced insulator-metal transition (IMT) of VO 2 thin films. It has been observed that the impedance matching-induced THz amplitude modulation was sensitive to the resistance switching characteristics of the VO 2 thin films. With four orders of change in resistance of the properly designed VO 2 films during the IMT, we experimentally achieved a near perfect THz modulator with an intensity modulation depth of 99.7 % between the insulator phase of VO 2 and the impedance matching state, and intensity modulation depth of 99.94% between the impedance matching state and the metallic phase of VO 2 . The experimental results were well explained by numerical simulations based on the transfer matrix model.

Monday, March 25, 2019

Abstract-Giant dual-mode graphene-based terahertz modulator enabled by Fabry–Perot assisted multiple reflection



Pei-Ren Tang, Jiang Li, Sen-Cheng Zhong, Zhao-Hui Zhai, Bing Zhu, Liang-Hui Du, Ze-Ren Li, Li-Guo Zhu

https://www.osapublishing.org/ol/abstract.cfm?uri=ol-44-7-1630

We report a high-performance terahertz (THz) modulator with dual operation mode. For the pulse operation mode, the proposed THz modulator has the advantage of high modulation depth (MD) and can operate in a broadband frequency range. We have experimentally achieved a MD larger than 90% for the fifth-order pulse THz echo at 0.8 THz, and the MD stays larger than 75% in a broadband frequency range larger than 1 THz, whereas, for the coherent operation mode, the Fabry–Perot (F-P) interference effect has been taken into consideration and a MD larger than 75% at 0.76 THz has also been realized.
© 2019 Optical Society of America

Wednesday, January 2, 2019

Abstract-Myelin Sheath as a Dielectric Waveguide for Signal Propagation in the Mid‐Infrared to Terahertz Spectral Range


Guozhi Liu,  Chao Chang,  Zhi Qiao,  Kaijie Wu,  Zhi Zhu,  Gangqiang Cui,   Wenyu Peng,  Yuzhao Tang,  Jiang Li, Chunhai Fan,

The myelin sheath, which serves as a dielectric waveguide for signal propagation, is experimentally confirmed using Fourier‐transform infrared microspectroscopy. The high contrast of reflectivity/refractivity between the myelin sheath and inner axon and outer medium at certain mid‐infrared to terahertz spectral range realize energy concentrates in myelin, and signal propagation is amplified when crossing the nodes of Ranvier via periodic relay.


https://onlinelibrary.wiley.com/doi/10.1002/adfm.201807862





The myelin sheath enables dramatic speed enhancement for signal propagation in nerves. In this work, myelinated nerve structure is experimentally and theoretically studied using synchrotron‐radiation‐based Fourier‐transform infrared microspectroscopy. It is found that, with a certain mid‐infrared to terahertz spectral range, the myelin sheath possesses a ≈2‐fold higher refraction index compared to the outer medium or the inner axon, suggesting that myelin can serve as an infrared dielectric waveguide. By calculating the correlation between the material characteristics of myelin and the radical energy distribution in myelinated nerves, it is demonstrated that the sheath, with a normal thickness (≈2 µm) and dielectric constant in nature, can confine the infrared field energy within the sheath and enable the propagation of an infrared signal at the millimeter scale without dramatic energy loss. The energy of signal propagation is supplied and amplified when crossing the nodes of Ranvier via periodic relay. These findings provide the first model for explaining the mechanism of infrared and terahertz neurotransmission through myelinated nerves, which may promote the development of biological‐tissue label‐free detection, biomaterial‐based sensors, neural information, and noninvasive brain–machine interfaces.

Sunday, December 23, 2018

Abstract-Terahertz wave near-field compressive imaging with a spatial resolution of over λ/100




Si-Chao Chen, Liang-Hui Du, Kun Meng, Jiang Li, Zhao-Hui Zhai, Qi-Wu Shi, Ze-Ren Li, and Li-Guo Zhu

https://www.osapublishing.org/ol/abstract.cfm?uri=ol-44-1-21

We demonstrate terahertz (THz) wave near-field imaging with a spatial resolution of 4.5μmusing single-pixel compressive sensing enabled by femtosecond-laser (fs-laser) driven vanadium dioxide (VO2)-based spatial light modulator. By fs-laser patterning a 180 nm thick VO2 nanofilm with a digital micromirror device, we spatially encode the near-field THz evanescent waves. With single-pixel Hadamard detection of the evanescent waves, we reconstructed the THz wave near-field image of an object from a serial of encoded sequential measurements, yielding improved signal-to-noise ratio by one order of magnitude over a raster-scanning technique. Further, we demonstrate that the acquisition time was compressed by a factor of over four with 90% fidelity using a total variation minimization algorithm. The proposed THz wave near-field imaging technique inspires new and challenging applications such as cellular imaging.
© 2018 Optical Society of America

Monday, November 12, 2018

Abstract-Ultrasensitive specific terahertz sensor based on tunable plasmon induced transparency of a graphene micro-ribbon array structure



Pei-ren Tang, Jiang Li, Liang-hui Du, Qiao Liu, Qi-xian Peng, Jian-heng Zhao, Bing Zhu, Ze-ren Li, Li-guo Zhu,

Fig. 1 Conceptual view of the PIT-sensor based on graphene micro-ribbon (GMR). The electromagnetic field is mainly concentrated at the edges of GMR, when excited by a THz wave, leading to the enhanced interaction between THz wave and the analyte. The tunability of the PIT sensor is achieved by changing the bias voltages (V1 and V2) applied on the two sets of GMR arrays.

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-26-23-30655

We proposed an ultrasensitive specific terahertz sensor consisting of two sets of graphene micro-ribbon with different widths. The interference between the plasmon resonances of the wide and narrow graphene micro-ribbons gives rise to the plasmon induced transparency (PIT) effect and enables ultrasensitive sensing in terahertz region. The performances of the PIT sensor have been analyzed in detail considering the thickness and refractive index sensing applications using full wave electromagnetic simulations. Taking advantage of the electrical tunability of graphene’s Fermi level, we demonstrated the specific sensing of benzoic acid with detection limit smaller than 6.35 µg/cm2. The combination of specific identification and enhanced sensitivity of the PIT sensor opens exciting prospects for bio/chemical molecules sensing in the terahertz region.
© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Tuesday, June 26, 2018

Abstract-Terahertz spectroscopy of neurodegenerative diseases: the correlation between terahertz biophysics and pathological analysis


Li-Guo Zhu, Yi Zou, Jiang Li, and Qiao Liu


https://www.osapublishing.org/abstract.cfm?uri=ISUPTW-2018-TuF4

·                                    The 9th International Symposium on Ultrafast Phenomena and Terahertz Waves

In this talk, I'll review and present our recent studies on THz spectroscopy of neurodegenerative diseased brain tissue and living cell. The well-matched correlation between THz biophysical properties and pathological analysis will also be discussed.
© 2018 OSA

Monday, December 18, 2017

Abstract-Label-free monitoring of cell death induced by oxidative stress in living human cells using terahertz ATR spectroscopy



Yi Zou, Qiao Liu, Xia Yang, Hua-Chuan Huang, Jiang Li, Liang-Hui Du, Ze-Ren Li, Jian-Heng Zhao, and Li-Guo Zhu

https://www.osapublishing.org/boe/abstract.cfm?uri=boe-9-1-14&origin=search

We demonstrated that attenuated total reflectance terahertz time-domain spectroscopy (ATR THz-TDS) is able to monitor oxidative stress response of living human cells, which is proven in this work that it is an efficient non-invasive, label-free, real-time and in situ monitoring of cell death. Furthermore, the dielectric constant and dielectric loss of cultured living human breast epithelial cells, and along with their evolution under oxidative stress response induced by high concentration of H2O2, were quantitatively determined in the work. Our observation and results were finally confirmed using standard fluorescence-labeled flow cytometry measurements and visible fluorescence imaging.
© 2017 Optical Society of America under the terms of the OSA Open Access Publishing 

Monday, July 10, 2017

Abstract-Dual-mode tunable terahertz generation in lithium niobate driven by spatially shaped femtosecond laser





Sen-Cheng Zhong, Yu Zhu, Liang-Hui Du, Zhao-Hui Zhai, Jiang Li, Jian-Heng Zhao, Ze-Ren Li, and Li-Guo Zhu

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-25-15-17066

A new approach for dual-mode (namely broadband mode and narrowband mode) terahertz (THz) pulses generation in a single lithium niobate (LN) crystal excited by spatially shaped tilted-pulse-front femtosecond (fs) laser pulse was proposed and experimentally demonstrated. The two THz emission modes are generated simultaneously while spatially separated. Both central frequency and bandwidth of narrowband THz emission is controllable by in situ tuning the spatial modulation period and beam size of the fs-laser, and the broadband (0.1-1.5 THz) THz emission keeps almost unchanged while tuning the narrowband emission. Further optimization achieves the narrowband THz emission with energy spectral density up to 0.27 μJ/THz and with bandwidth narrowly down to 23 GHz. Such dual-mode THz source is useful for nonlinear THz optics, such as selected resonant THz excitation with broadband THz probe spectroscopy of crystalline matters.
© 2017 Optical Society of America

Monday, November 23, 2015

Abstract-Optimization of terahertz generation from LiNbO3 under intense laser excitation with the effect of three-photon absorption


Sen-Cheng Zhong, Zhao-Hui Zhai, Jiang Li, Li-Guo Zhu, Jun Li, Kun Meng, Qiao Liu, Liang-Hui Du, Jian-Heng Zhao, and Ze-Ren Li
https://www.osapublishing.org/oe/abstract.cfm?uri=oe-23-24-31313
We proposed a three-dimensional model to simulate terahertz generation from LiNbO3crystal under intense laser excition (up to ~50 mJ/cm2). The impact of three-photon absorption, which leads to free carrier generation and free carrier saturation (when pump fluence above ~10 mJ/cm2) on terahertz generation was investigated. And further with this model, we stated the optimized experimental conditions (incident postion, beam diameter, and pulse duration, etc) for maximum generation efficiency in commonly-used tilted-pulse-front scheme. Red shift of spectrum, spatial distribution “splitting” effects of emitted THz beam, and primilary experimental verification under intense laser excitation are given.
© 2015 Optical Society of America
Full Article  |  PDF Article

Friday, July 18, 2014

Future electronics may depend on lasers, not quartz



Vahala's new laser frequency reference (left) is a small 6 mm disk; the quartz "tuning fork" (middle) is the frequency reference commonly used today in wristwatches to set the second. The dime (right) is for scale. Credit: Jiang Li/Caltech

by Jessica Stoller-Conrad
:http://phys.org/news/2014-07-future-electronics-lasers-quartz.html#jCp

(Phys.org) —Nearly all electronics require devices called oscillators that create precise frequencies—frequencies used to keep time in wristwatches or to transmit reliable signals to radios. For nearly 100 years, these oscillators have relied upon quartz crystals to provide a frequency reference, much like a tuning fork is used as a reference to tune a piano. However, future high-end navigation systems, radar systems, and even possibly tomorrow's consumer electronics will require references beyond the performance of quartz.

Now, researchers in the laboratory of Kerry Vahala, the Ted and Ginger Jenkins Professor of Information Science and Technology and Applied Physics at Caltech, have developed a method to stabilize  in the range of gigahertz, or billions of cycles per second—using a pair of laser beams as the reference, in lieu of a crystal.

Quartz crystals "tune" oscillators by vibrating at relatively low frequencies—those that fall at or below the range of megahertz, or millions of cycles per second, like radio waves. However, quartz crystals are so good at tuning these low frequencies that years ago, researchers were able to apply a technique called electrical frequency division that could convert higher-frequency microwave signals into lower-frequency signals, and then stabilize these with quartz.
The new technique, which Vahala and his colleagues have dubbed electro-optical frequency division, builds off of the method of optical frequency division, developed at the National Institute of Standards and Technology more than a decade ago. "Our new method reverses the architecture used in standard crystal-stabilized microwave oscillators—the 'quartz' reference is replaced by optical signals much higher in frequency than the microwave signal to be stabilized," Vahala says.
Jiang Li—a Kavli Nanoscience Institute postdoctoral scholar at Caltech and one of two lead authors on the paper, along with graduate student Xu Yi—likens the method to a gear chain on a bicycle that translates pedaling motion from a small, fast-moving gear into the motion of a much larger wheel. "Electrical frequency dividers used widely in electronics can work at frequencies no higher than 50 to 100 GHz. Our new architecture is a hybrid electro-optical 'gear chain' that stabilizes a common microwave electrical oscillator with optical references at much higher frequencies in the range of terahertz or trillions of cycles per second," Li says.
The optical reference used by the researchers is a laser that, to the naked eye, looks like a tiny disk. At only 6 mm in diameter, the device is very small, making it particularly useful in compact photonics devices—electronic-like devices powered by photons instead of electrons, says Scott Diddams, physicist and project leader at the National Institute of Standards and Technology and a coauthor on the study.
"There are always tradeoffs between the highest performance, the smallest size, and the best ease of integration. But even in this first demonstration, these optical oscillators have many advantages; they are on par with, and in some cases even better than, what is available with widespread electronic technology," Vahala says.
The new technique is described in a paper that will be published in the journal Science on July 18.
More information: Electro-optical frequency division and stable microwave synthesis, Science 18 July 2014: Vol. 345 no. 6194 pp. 309-313 . DOI: 10.1126/science.1252909


Read more at: http://phys.org/news/2014-07-future-electronics-lasers-quartz.html#jCp