Showing posts with label János Hebling. Show all posts
Showing posts with label János Hebling. Show all posts

Tuesday, December 17, 2019

Abstract-Matter manipulation with extreme terahertz light: Progress in the enabling THz technology



Peter Salén,  Martina Basini, Stefano Bonetti, János Hebling, Mikhail Krasilnikov, Alexey Y. Nikitin, Georgii Shamuilov, Zoltán Tibai, Vitali Zhaunerchyk, Vitaliy Goryashko, 


Fig. 1. (a) Fundamental excitations in solids and molecular systems in the THz regionFig. 5. (a) Transient reflectance of the stripe-ordered cuprate LESCO1∕8

https://www.sciencedirect.com/science/article/pii/S0370157319302649

Terahertz (THz) light has proven to be a fine tool to probe and control quasi-particles and collective excitations in solids, to drive phase transitions and associated changes in material properties, and to study rotations and vibrations in molecular systems. In contrast to visible light, which usually carries excessive photon energy for collective excitations in condensed matter systems, THz light allows for direct coupling to low-energy (meV scale) excitations of interest. The development of light sources of strong-field few-cycle THz pulses in the 2000s opened the door to controlled manipulation of reactions and processes. Such THz pulses can drive new dynamic states of matter, in which materials exhibit properties entirely different from that of the equilibrium. In this review, we first systematically analyze known studies on matter manipulation with strong-field few-cycle THz light and outline some anticipated new results. We focus on how properties of materials can be manipulated by driving the dynamics of different excitations and how molecules and particles can be controlled in useful ways by extreme THz light. Around 200 studies are examined, most of which were done during the last five years. Secondly, we discuss available and proposed sources of strong-field few-cycle THz pulses and their state-of-the-art operation parameters. Finally, we review current approaches to guiding, focusing, reshaping and diagnostics of THz pulses.

Saturday, March 16, 2019

Abstract-Numerical investigation of imaging-free terahertz generation setup using segmented tilted-pulse-front excitation




György Tóth, László Pálfalvi, József A. Fülöp, Gergő Krizsán, Nicholas H. Matlis, Gábor Almási, and János Hebling

Fig. 1 The setup of the investigated hybrid NLES THz source. The dark blue lines represent the pump pulse front at different moments. After diffraction of the pump beam on the transmission grating (TG), it propagates horizontally. Consequently, the phase-fronts are vertical. All γ is measured from a vertical line.


https://www.osapublishing.org/oe/abstract.cfm?uri=oe-27-5-7762

Recently a hybrid-type terahertz (THz) pulse source was proposed for high energy terahertz pulse generation. It is the combination of the conventional tilted-pulse-front setup and a nonlinear crystal with a transmission stair-step echelon of period in the hundred-micrometer range etched into the front face. The tilt angle introduced by the conventional tilted-pulse-front setup (pre-tilt) was chosen to be equal to the tilt-angle needed inside the nonlinear crystal (62° for lithium niobate (LN)) in order to fulfill velocity-matching. In this case, plane-parallel nonlinear optical crystals can be used. The possibility of using a plane-parallel nonlinear optical crystal for producing good-quality, symmetric THz beams was considered the most important advantage of this setup. In the present paper, a thorough numerical investigation of a modified version of that setup is presented. In the new version, the tilted pulse-front is created by a transmission grating without any imaging optics, and a wedged nonlinear optical crystal with a small wedge angle is supposed. According to a 1D numerical code, significantly higher THz generation efficiency can be achieved with a transmission stair-step echelon-faced nonlinear crystal having a 5 – 15-degree wedge angle than with a plane-parallel one or with the conventional tilted-pulse-front setup. Because of the spatially-dependent group-delay dispersion introduced by the transmission grating, a small wedge in the nonlinear crystal improves the spatial homogeneity of the THz-generation process, resulting in higher efficiencies and better beam profiles. At 100 K temperature, and by using 800 nm pump pulses with 20 mJ pulse energy, 100 fs pulse length and 8 mm beam spot radius, approximately 4.5% conversion efficiency and close to 1 mJ terahertz pulse energy can be reached with the newly-proposed setup.
© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Saturday, September 1, 2018

Abstract-Demonstration of a Tilted-Pulse-Front Pumped Plane-Parallel Slab Terahertz Source




A new type of tilted-pulse-front pumped terahertz (THz) source has been demonstrated, which is based on a lithium niobate plane-parallel slab with an echelon structure on its input surface. Single-cycle pulses of 1 microjoule energy and 0.30 THz central frequency have been generated with 0.05% efficiency from such a source. One order-of-magnitude increase in efficiency is expected by pumping a cryogenically cooled echelon of increased size and thickness with a Ti:sapphire laser. The use of a plane-parallel nonlinear optical crystal slab enables straightforward scaling to high THz pulse energies and to produce a symmetric THz beam with uniform pulse shape for good focusability and high field strength.

Sunday, April 22, 2018

Abstract-Single-cycle attosecond pulses by Thomson backscattering of terahertz pulses



György Tóth, Zoltán Tibai, Ashutosh Sharma, József A. Fülöp, and János Hebling

https://www.osapublishing.org/josab/abstract.cfm?uri=josab-35-5-A103

The generation of single-cycle attosecond pulses based on Thomson scattering of terahertz (THz) pulses is proposed. In the scheme, a high-quality relativistic electron beam, produced by a laser-plasma wakefield accelerator, is sent through suitable magnetic devices to produce ultrathin electron layers for coherent Thomson backscattering of intense THz pulses. According to numerical simulations, single-cycle attosecond pulse generation is possible with up to 1 nJ energy. The waveform of the attosecond pulses closely resembles that of the THz pulses. This allows for flexible waveform control of attosecond pulses.
© 2018 Optical Society of America

Saturday, April 14, 2018

Abstract-Scalable Concepts for THz Generation by Tilted-Pulse-Front Pumping


Jozsef A. Fulop, László Pálfalvi, Gyorgy Toth, Gyula Polónyi, Balázs Monoszlai, Levente Tokodi, Gábor Almási, and János Hebling

https://www.osapublishing.org/abstract.cfm?uri=HILAS-2018-HT3A.1

A monolithic contact-grating semiconductor source and a hybrid LiNbO3stair-step echelon are presented for efficient THz pulse generation by optical rectification. They enable excellent focusability of the THz beams and are scalable to mJ-level THz pulse energies.
© 2018 OSA

Thursday, April 5, 2018

Abstract-Intense terahertz sources for nonlinear interactions


 József A. Fülöp,  László Pálfalvi,   János Hebling,

http://ieeexplore.ieee.org/document/8105130/


The present status and the prospects of efficient pulsed terahertz (THz) sources based on optical rectification in lithium niobate and semiconductors, pumped by femtosecond pulses with tilted intensity front, will be discussed. Applications range from nonlinear THz spectroscopy and multispectral imaging to electron and proton acceleration.

Monday, April 2, 2018

Abstract-Dual-chirped optical parametric amplifier for pumping multicycle tunable terahertz pulse source


Gyorgy Toth, Jozsef A. Fulop, and János Hebling

https://www.osapublishing.org/search.cfm?q=terahertz&meta=1&cj=1&cc=1

DC-OPA is proposed for generation of periodically intensity-modulated-pulses by interference of the signal and the idler. These pulses allows to tunable THz-pulse generation by the chirp and the delay between the pump and the signal.
© 2018 OSA

Monday, November 27, 2017

Abstract-Single-cycle attosecond pulses by Thomson backscattering of terahertz pulses



The generation of single-cycle attosecond pulses based on Thomson scattering of terahertz (THz) pulses is proposed. In the scheme, a high-quality relativistic electron beam produced by a laser-plasma wakefield accelerator (LPWA), is sent through suitable magnetic devices to produce ultrathin electron layers for coherent Thomson backscattering of intense THz pulses. According to numerical simulations, single-cycle attosecond pulse generation is possible with up to 1 nJ energy. The waveform of the attosecond pulses closely resembles that of the THz pulses. This allows for a flexible waveform control of attosecond pulses.

Thursday, November 23, 2017

Abstract-Numerical investigation of a scalable setup for efficient terahertz generation using a segmented tilted-pulse-front excitation



László Pálfalvi, György Tóth, Levente Tokodi, Zsuzsanna Márton, József András Fülöp, Gábor Almási, and János Hebling

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-25-24-29560v


A hybrid-type terahertz pulse source is proposed for high energy terahertz pulse generation. It is the combination of the conventional tilted-pulse-front setup and a transmission stair-step echelon-faced nonlinear crystal with a period falling in the hundred-micrometer range. The most important advantage of the setup is the possibility of using plane parallel nonlinear optical crystal for producing good-quality, symmetric terahertz beam. Another advantage of the proposed setup is the significant reduction of imaging errors, which is important in the case of wide pump beams that are used in high energy experiments. A one dimensional model was developed for determining the terahertz generation efficiency, and it was used for quantitative comparison between the proposed new hybrid setup and previously introduced terahertz sources. With lithium niobate nonlinear material, calculations predict an approximately ten-fold increase in the efficiency of the presently described hybrid terahertz pulse source with respect to that of the earlier proposed setup, which utilizes a reflective stair-step echelon and a prism shaped nonlinear optical crystal. By using pump pulses of 50 mJ pulse energy, 500 fs pulse length and 8 mm beam spot radius, approximately 1% conversion efficiency and 0.5 mJ terahertz pulse energy can be reached with the newly proposed setup.

© 2017 Optical Society of America

Saturday, November 4, 2017

Abstract-Periodically intensity-modulated pulses by optical parametric amplification for multicycle tunable terahertz pulse generation




György Tóth, József A. Fülöp, and János Hebling

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-25-23-28258

The superposition of signal and idler pulses in dual-chirped optical parametric amplification is proposed for the efficient generation of intensity-modulated pulses with periodic modulation. Both the duration and the modulation period are easily and independently adjustable. Numerical simulations for a three-stage optical parametric amplifier system predicted an efficiency as high as ~50% for about 40 mJ of output pulse energy at a wavelength of 2 µm. Sources of such intensity-modulated pulses near 1.6 µm or 2 µm wavelength, pumped by Ti:sapphire or Yb-doped lasers, can be ideally suited for intense multicycle THz pulse generation with tunable frequency and bandwidth by optical rectification for example in organic, semiconductor, or lithium niobate materials.
© 2017 Optical Society of America

Thursday, May 11, 2017

Abstract-Refractive Index and Absorption Coefficient of Undoped and Mg-Doped Lithium Tantalate in the Terahertz Range


Andrea Buzády, Márta Unferdorben, György Tóth, János Hebling, Ivett Hajdara, László Kovács, László Pálfalvi

https://link.springer.com/article/10.1007%2Fs10762-017-0393-y

Dielectric material parameters of lithium tantalate (LT) in the terahertz region have been investigated using terahertz time-domain spectroscopy (THz-TDS). Undoped congruent, undoped stoichiometric, and Mg-doped stoichiometric LT crystals were measured. The Mg content was 0.5 and 1.0 mol% for the stoichiometric composition. Index of refraction and absorption coefficient spectra were determined in the 0.3–2.0-THz frequency range for beam polarization both parallel (extraordinary polarization) and perpendicular (ordinary polarization) to the optical axis [001] of the crystal at room temperature. For the calculation of the refractive index and absorption coefficient spectra from the measured data, we used TeraMat software (Menlo System) belonging to the spectrometer. The refractive index and the absorption coefficient for stoichiometric crystals were lower than for the congruent one. In the case of stoichiometric crystals, the Mg dopant caused a slight reduction of both ordinary and extraordinary refractive index compared to the undoped crystal. However, the presence of Mg did not reduce the absorption coefficient either for the ordinary or for the extraordinary polarization. In order to fit the measurement data, a Lorentz oscillator model was used. Good agreement was obtained between the measured data and the fitting curves by using the Lorentz oscillator model containing three terms.

Tuesday, May 26, 2015

Abstract-Measurement of Refractive Index and Absorption Coefficient of Congruent and Stoichiometric Lithium Niobate in the Terahertz Range







Time domain THz spectroscopy measurements were performed on a series of undoped and Mg-doped congruent lithium niobate crystals with 1.2, 6.1, and 8.4 mol% Mg concentrations and on undoped and Mg-doped stoichiometric lithium niobate crystals with 0.7, 1.5, and 4.2 mol% Mg concentrations with polarization parallel (extraordinary) and perpendicular (ordinary) to the z axis of the crystal at 300 K. The absorption coefficient and refractive index spectra were determined in theTHz frequency range from 0.25 to ~2.5 THz. In the case of congruent samples for both polarizations, both the refractive index and the absorption coefficient have minimal values for compositions close to the photorefractive threshold. In the case of stoichiometric samples, similar tendencies close to the photorefractive threshold at lower Mg concentration were observed but only for extraordinary polarization, while for ordinary polarization the measured values, especially for the absorption coefficient, were only weakly dependent on the Mg content.

Tuesday, December 20, 2011

THz pulse technology brings new hope to cancer patients




http://networkedblogs.com/rOzqH
A team of scientists from the University of Pécs who developed a method for producing ultra-short high-energy terahertz pulses, are now confident that they will be able to increase the electric field value of these pulses by a magnitude of 100. This development could lead to a variety of new and exciting applications, ranging from cancer therapy to semiconductor research. We spoke to János Hebling and József Fülöp to find out more.
Terahertz radiation is a specific type of electromagnetic radiation that lies between the frequency ranges of microwave and infrared radiation. Around 25 years ago, scientists began investigating the use of femtosecond laser pulses for the generation of THz radiation, resulting in the generation of THz pulses with a frequency one to three orders of magnitude larger than any electronic device can produce. Using this technique, THz pulses comprised of only a single oscillation of the electric field can be obtained (see Figure on next page).
THz radiation has a number of useful applications, such as for security devices in airports. It is able to penetrate through most materials that are used for packaging, so by using multispectral THz imaging, dangerous substances such as biological weapons or drugs can be detected without having to open the packaging. It is also able to do this incredibly quickly, making it extremely practical.
Professor János Hebling, director of the Institute of Physics at the University of Pécs explains how he first became involved in THz research: “Back in 2000, I was working at the Max Planck institute in Stuttgart where I was investigating the temporal behaviour of phonon polaritons in semiconductors. I developed a novel setup for the generation of such excitations using ultra-short laser pulses.
“When I later began work at the University of Pécs, we realised that we could use this setup for the generation of high-energy THz pulses using nonlinear materials such as lithium-niobate.”
Nonlinear optical materials are materials in which the electric field of light output is not related to the electric field of light input by a simple proportionality constant. Because of this nonlinear behaviour, an intense light beam propagating through a nonlinear optical material can produce new frequency components not contained in the input light, which cannot be seen with weak light beams.
For example, an intense light beam propagating through a nonlinear material can generate, in addition, harmonics or overtones of the original light frequency such as its second harmonic, used also in green laser pointers. The difference of two input frequency components can also be generated if the velocity of the input laser radiation and that of the generated low-frequency (THz) radiation are equal. In lithium-niobate, a highly nonlinear material, this can be accomplished by tilting the intensity front of the input short laser pulses. Ultrashort laser pulses can be said to be like flying pancakes, since their spatial extension in the direction of propagation is very small. Hence, tilting the intensity front means a slanted flying pancake. This technique of tilted-pulse-front pumping developed by the team in Pécs is now used by several groups around the world for THz pulse generation.
“By using high pump pulse energies, we were able to generate incredibly intense THz pulses, which we then used in the first THz pump—THz probe experiments at MIT, Cambridge,” continues Hebling. “This method of THz generation is now used widely by research groups from around the world.”
Only a few years ago, an electric field value of 1 MV/cm was considered very high, but it has been predicted that field strengths as high as 100 MV/cm are possible in the future. This would be achieved with a modified setup by using longer pump pulses and cooling the lithium-niobate crystals to very low temperatures. This could allow for a number of exciting new applications, including the manipulation of ions and relativistic electrons.
Jozsef Fülöp, another member of the team, further explains what the implications of their THz research are: “I was very keen to get involved in the development of this project, as it was clear that in the future there were a lot of things that could be done with this technology.
“We are now at a stage where some of these applications, such as non-linear THz spectroscopy, have started to be demonstrated. In the last two years we have seen that these pulses can introduce changes in the state of charged carriers in semiconductors, and they do this instantaneously because they are very short. This will help for a better understanding of ultrafast carrier dynamics of electron distribution in these materials, which will have applications in electronics.”
“One of the most interesting uses that we envisage for the future is the manipulation of charged particles, for instance the acceleration of electrons and protons,” he continues. “This could eventually be used for medical applications such as cancer therapy.”
This sort of radiation therapy for treating cancer using ion beams is known as particle therapy, or more accurately, hadron therapy. This works by aiming beams of energetic hadrons, i.e. protons or ions, at a tumor. The main reason why ion beams are superior to x-ray or gamma radiation in cancer therapy is their different absorption characteristics. Ion beams are mainly absorbed at a well defined depth inside the tissue, while hardly effecting the tissue outside of this depth. Gamma rays follow the usual exponential attenuation law, therefore they are mainly absorbed close to the surface, thereby heavily damaging the healthy tissue outside the tumor.
The team from Pécs has submitted a number of patents for the use of high field strength THz pulses for this application, and so hopefully in the future their research into this field could lead to reducing the suffering of cancer patients around the world.
Source: Projects Magazine.