Showing posts with label Claudia Gollner. Show all posts
Showing posts with label Claudia Gollner. Show all posts

Wednesday, May 13, 2020

IR Laser Mixing, Optical “Magic” Yields THz Waves with Relative Efficiency



By mixing and manipulating an infrared laser, a team led by researchers at TU Wein (Vienna University of Technology) has generated a wide band of terahertz waves with relatively high efficiency.

The terahertz segment of the electromagnetic spectrum exists in a sort of “twilight zone” between about 300 GHz (0.3 THz) to 3 THz (note that the upper boundary value is somewhat arbitrary, and some consider it to be 30 THz). It’s bounded below by millimeter-wave RF (30 to 300 GHz) and above by optical wavelengths. Electromagnetic radiation below the terahertz band can be created by many sources and emitted by antennas, while the optical radiation above the terahertz band can be developed by solid-state lasers.

However, the major part of the terahertz span is largely a void. Although it’s governed by Maxwell’s equations just as the rest of the spectrum, it’s relatively difficult to generate these waves as they’re too high in frequency for even most leading-edge electronic components and too low for optical sourcing. Due to this and other problems, the terahertz region is far less explored and exploited than the RF or optical areas (see “References” at end of article).
Why even investigate the terahertz part of the spectrum? Among the many reasons are because it’s there, of course; because it potentially has useful and fascinating characteristics; and it may be needed for 6G, 7G, or 8G wireless links. After all, 20 years ago, if you had told someone that there would be mass-market consumer products operating at ~10 GHz by the first part of the 21st century, you would have likely been called a wild-eyed dreamer.
Power Problems
However, the problem remains in terms of efficiently generating useful levels of power in the terahertz band. There are tabletop sources based on either optical rectification in electro-optic crystals or two-color filamentation in gases and liquids. With optical rectification, terahertz pulses with energy up to 0.9 mJ and THz conversion efficiency (ratio of generated THz energy to the input laser pulse energy) up to 3.7% have been generated, but the pulses are long (several picoseconds) with narrow spectra.
Unfortunately, the optical-damage threshold of electro-optic crystals prevents a significant increase in power. Furthermore, while there are no issues with optical damage when using the two-color filamentation approach, it generates only less-energetic near-infrared (NIR) laser pulses, and with a very low conversion efficiency of ~0.01%.
Efficient Source Breakthrough
Now, a research group based at TU Wein (Vienna University of Technology), in close cooperation with a team from the Institute of Electronic Structure and Laser (IESL) Foundation for Research and Technology-Hellas (FORTH) in Heraklion, Greece, and some help from Texas A&M University at Qatar, has developed a source that’s both fairly efficient and can generate waves across the entire terahertz slice of spectrum. The experiment, with results they claim has broken previous records in these areas, was inspired by a theory developed in Texas A&M University, which predicted that long-wavelength laser pulses could be used to achieve extremely efficient terahertz generation in air plasma.
In the setup schematic (Fig. 1), the generation of the terahertz waves begins by sending infrared laser light through a nonlinear medium, where part of the infrared radiation is transformed into optical radiation at twice the initial frequency. The two radiation waves are then superimposed, creating an electromagnetic wave with an electric field having a very specific asymmetric shape.
The setup for THz generation by two-color mid-infrared filaments (a). After the quarter wave plate (QWP), the 3.9-μm laser pulse passes through the gallium-selenide (GaSe) crystal and generates the second harmonic pulse. The two-color laser pulse is focused by an off-axis parabolic mirror (OPM1) in ambient air and forms a filament where the THz radiation is generated. A parabolic mirror (OPM2) gathers the emitted THz pulse and guides it into one of the detection setups. The metallic disk (MD) blocks the on-axis mid-infrared radiation and generated supercontinuum, while the conically emitted THz radiation passes around it. A set of lowpass filters filter out the remained unwanted radiation and prevent the saturation of the pyroelectric detector (PED) by the intense THz pulses. THz detection setups (b-d): The parabolic mirror (OPM3) focuses the THz pulse on the PED to measure its energy (b). The wire grid polarizer (GP), placed before the OPM3, makes it possible to characterize the THz polarization. For the electro-optic measurements, the parabolic mirror (OPM4) focuses the THz pulse into a 55-μm thick gallium phosphide (GaP) crystal (c). A pair of GPs reduces the THz field strength to ensure a linear response. The 680-nm synchronized probe pulse focuses into the GaP crystal through a hole in OPM4 and then is guided to the balanced detection setup. For the cross-phase modulation experiment, the GaP crystal is replaced by the 1-mm-thick zinc-telluride (ZnTe) crystal and the 761-nm probe pulse is guided to the spectrometer. The Michelson interferometer measures the THz field autocorrelation and consists of a pellicle beam splitter (PBS) and two flat mirrors: fixed (M1) and movable (M2) (d). At the exit, a parabolic mirror (OPM5) focuses the radiation on the PED. (Source: TU Wein)

But that’s only the start of this process. The intense wave “rips” electrons out of the molecules in the air, turning the air into a glowing plasma. The special shape of the wave's electric field accelerates the electrons in such a way that they produce the desired terahertz radiation.
As noted by team member Claudia Gollner (Fig. 2), “Our method is extremely efficient with 2.3% of the supplied energy converted into terahertz radiation. That is orders of magnitude more than can be achieved with other methods. This results in exceptionally high terahertz energies of almost 200 microjoules and terahertz-field amplitudes exceeding 100 MV per cm.”
Researcher Claudia Gollner adjusts the optoelectronic setup in the lab at TU Wein’s photonics institute. (Source: TU Wein)
She also added that their approach develops many wavelengths throughout the terahertz range to be emitted simultaneously, and the larger spectrum of different terahertz wavelengths yields the shorter and more intense pulses.
The details, including a review of existing methods of terahertz generation and their characteristics, are in their paper “Observation of extremely efficient terahertz generation from mid-infrared two-color laser filaments” published in Nature Communications, along with even-more detailed, equation-laced Supplementary Information.
References
IEEE Spectrum, “The Truth About Terahertz

Tuesday, January 21, 2020

Record-breaking terahertz laser beam




Claudia Gollner and her laser system. Credit: Vienna University of Technology
https://phys.org/news/2020-01-record-breaking-terahertz-laser.html

Terahertz radiation is used for security checks at airports, for medical examinations and also for quality checks in industry. However, radiation in the terahertz range is extremely difficult to generate. Scientists at TU Wien have now succeeded in developing a terahertz radiation source that breaks several records: it is extremely efficient, and its spectrum is very broad—it generates different wavelengths from the entire terahertz range. This opens up the possibility of creating short radiation pulses with extremely high radiation intensity. The new terahertz technology has now been presented in the journal Nature Communications.
The "Terahertz Gap" Between Lasers and Antennas
"Terahertz  has very useful properties," says Claudia Gollner from the Institute of Photonics at TU Wien. "It can easily penetrate many materials, but unlike X-rays, it is harmless because it is not ionizing radiation."
From a technical point of view, however,  radiation is located in a frequency region which is very hard to access—in sort of a no man's land between two well-known areas: Radiation with higher frequencies can be generated by ordinary solid-state lasers. Low-frequency radiation, on the other hand, as it is used in mobile communications, is emitted by antennas. The greatest challenges lie exactly in between, in the terahertz range.
In the laser laboratories of TU Wien, a great deal of effort must therefore be put into generating the desired high-intensity terahertz radiation pulses. "Our starting point is the radiation of an infrared laser system. It was developed at our Institute and it is unique in the world," says Claudia Gollner. First, the laser light is sent through a so-called non-linear medium. In this material, the infrared radiation is modified, part of it is converted into radiation with twice the frequency.
"So now we have two different types of infrared radiation. These two kinds of radiation are then superimposed. This creates a wave with an electric field with a very specific asymmetric shape," says Gollner.
Turning Air into Plasma
This  is intense enough to rip electrons out of the molecules in the air. The air turns into a glowing plasma. Then, the special shape of the wave's  accelerates the electrons in such a way that they produce the desired terahertz radiaton.
"Our method is extremely efficient: 2.3% of the supplied energy is converted into terahertz radiation—that is orders of magnitude more than can be achieved with other methods. This results in exceptionally high THz energies of almost 200 µJ," says Claudia Gollner. Another important advantage of the new method is that a very broad spectrum of terahertz radiation is generated. Very different wavelengths throughout the  are emitted simultaneously. This produces extremely intense short radiation pulses. The larger the spectrum of different terahertz wavelengths, the shorter and more intense pulses can be generated.
Numerous Possible Applications
"This means that for the first time a terahertz source for extremely high intensity radiation is now available," says Andrius Baltuska, the head of the research group at the Vienna University of Technology. "Initial experiments with zinc-telluride crystals already show that  is excellently suited to answer important questions from material science in a completely new way. We are convinced that this method has a great future."

Saturday, January 18, 2020

Abstract-Terahertz response of gadolinium gallium garnet (GGG) and gadolinium scandium gallium garnet (SGGG)




We report the magneto-optical response of Gadolinium Gallium Garnet (GGG) and Gadolinium Scandium Gallium Garnet (SGGG) at frequencies ranging from 300GHz to 1THz, and determine the material response tensor. Within this frequency window, the materials exhibit nondispersive and low-loss optical responses. At low temperatures, significant THz Faraday rotations are found in the (S)GGG samples. Such strong gyroelectric response is likely associated with the high-spin paramagnetic state of the Gd3+ ions. A model of the material response tensor is determined, together with the Verdet and magneto-optic constants.

Abstract-Observation of extremely efficient terahertz generation from mid-infrared two-color laser filaments


https://www.nature.com/articles/s41467-019-14206-x

Extreme nonlinear interactions of THz electromagnetic fields with matter are the next frontier in nonlinear optics. However, reaching this frontier in free space is limited by the existing lack of appropriate powerful THz sources. Here, we experimentally demonstrate that two-color filamentation of femtosecond mid-infrared laser pulses at 3.9 μm allows one to generate ultrashort sub-cycle THz pulses with sub-milijoule energy and THz conversion efficiency of 2.36%, resulting in THz field amplitudes above 100 MV cm−1. Our numerical simulations predict that the observed THz yield can be significantly upscaled by further optimizing the experimental setup. Finally, in order to demonstrate the strength of our THz source, we show that the generated THz pulses are powerful enough to induce nonlinear cross-phase modulation in electro-optic crystals. Our work paves the way toward free space extreme nonlinear THz optics using affordable table-top laser systems.