Abstract-Quantum-inspired terahertz spectroscopy with visible photons

 

Mirco Kutas, Björn Haase, Jens Klier, Daniel Molter, and Georg von Freymann

Experimental setup. The 1 mm long PPLN crystals are pumped by a continuous-wave laser with a wavelength of 660 nm, generating correlated pairs of signal and terahertz photons. After the crystal the terahertz radiation is separated by an OAP with a through hole and afterwards reflected at a moveable mirror Mi. Pump and generated signal photons are reflected at Ms directly back into the crystal. After the second pass the pump radiation is filtered from the signal radiation by three volume Bragg gratings (VBGs). To obtain a frequency-angular spectrum on the sCMOS camera, the signal radiation is focused through a transmission grating (TG).

https://www.osapublishing.org/optica/fulltext.cfm?uri=optica-8-4-438&id=449480

Terahertz technology offers solutions in nondestructive testing and spectroscopy for many scientific and industrial applications. While direct detection of photons in this frequency range is difficult to achieve, quantum optics provides a highly attractive alternative: it enables the characterization of materials in hardly accessible spectral ranges by measuring easily detectable photons of a different spectral range. Here we report on the application of this principle to terahertz spectroscopy, measuring absorption features of chemicals at sub-terahertz frequencies by detecting visible photons. To generate the needed correlated signal-idler photon pairs, a periodically poled lithium niobate crystal and a 660 nm continuous-wave pump source are used. After propagating through a single-crystal nonlinear interferometer, the pump photons are filtered by narrowband volume Bragg gratings. An uncooled scientific CMOS camera detects the frequency-angular spectra of the remaining visible signal and reveals terahertz-spectral information. Neither cooled detectors nor expensive pulsed lasers for coherent detection are required.

© 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

Abstract-Terahertz quantum sensing

 Björn Haase, Daniel Molter, Felix Riexinger, Mirco Kutas, Patricia Bickert,

https://advances.sciencemag.org/content/6/11/eaaz8065

Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: Sample information is gained in the spectral region of interest and transferred via biphoton correlations into another spectral range, for which highly sensitive detectors are available. This is especially beneficial for terahertz radiation, where no semiconductor detectors are available and coherent detection schemes or cryogenically cooled bolometers have to be used. Here, we report on the first demonstration of quantum sensing in the terahertz frequency range in which the terahertz photons interact with a sample in free space and information about the sample thickness is obtained by the detection of visible photons. As a first demonstration, we show layer thickness measurements with terahertz photons based on biphoton interference. As nondestructive layer thickness measurements are of high industrial relevance, our experiments might be seen as a first step toward industrial quantum sensing applications.

Abstract-Terahertz Quantum Sensing

Mirco Kutas, Björn Haase, Patricia Bickert, Felix Riexinger, Daniel Molter, Georg von Freymann

https://arxiv.org/abs/1909.06855

Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: sample information is gained in the spectral region of interest and transferred via entanglement into another spectral range, for which highly sensitive detectors are available. This is especially beneficial for terahertz radiation, as the corresponding photon energy lies in the range of a few meV - an energy where no semiconductor detectors are available and coherent detection schemes or cryogenically cooled bolometers have to be employed. Here, we report on the first demonstration of quantum sensing in the terahertz frequency range in which the terahertz photons interact with a sample in free space and information about the sample thickness is obtained by the detection of visible photons. A nonlinear single-crystal interferometer setup with a periodically poled lithium niobate crystal (PPLN) and a 660 nm pump source is used, generating visible (signal) photons and associated (idler) photons in the terahertz frequency range. Separation from the pump photons and detection of the visible signal photons is achieved by using highly efficient and narrowband volume Bragg gratings and an uncooled scientific complementary metal-oxide-semiconductor (sCMOS) camera. The acquired frequency-angular spectra show quantum interference in the Stokes as well as the Anti-Stokes part of collinear forward generation caused by spontaneous parametric down-conversion (SPDC) and down-conversion as well as up-conversion of thermal photons. The information encoded in the quantum interference can be used to determine the thickness of coatings or functional layers that are mainly transparent in the terahertz spectral range. As a first demonstration, we show layer thickness measurements with terahertz photons based on induced coherence without induced emission.

Abstract-Spontaneous parametric down-conversion of photons at 660 nm to the terahertz and sub-terahertz frequency range

Björn Haase, Mirco Kutas, Felix Riexinger, Patricia Bickert, Andreas Keil, Daniel Molter, Michael Bortz, and Georg von Freymannark

Fig. 1 Phase-matching schemes. The periodic poling of the nonlinear crystal leads to a k-vector component kΛ, which can have two directions. This yields phase-matched terahertz generation in forward and backward direction. Pump (p), signal (s) and idler (THz) wave vectors have to be considered as non-collinear in down- (sd) and up-conversion (su).

https://www.osapublishing.org/oe/abstract.cfm?uri=oe-27-5-7458

We report on spontaneous parametric down-conversion (SPDC) in periodically poled lithium niobate (PPLN) using 660 nm pump wavelength and the type 0 phase-matching condition to the terahertz and even sub-terahertz frequency range. Detection of the frequency-shifted signal photons is achieved by using highly efficient and narrowband volume Bragg gratings and an uncooled sCMOS camera. The acquired frequency-angular spectrum shows backward and forward generation of terahertz and sub-terahertz photons by SPDC, as well as up-conversion and higher order quasi phase-matching (QPM). The frequency-angular spectrum is theoretically calculated using a Monte-Carlo integration scheme showing a high agreement with the measurement. This work is one important step toward quantum sensing and imaging in the terahertz and sub-terahertz frequency range.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement